Spatiotemporal control for integrated catalysis
Spatiotemporal control for integrated catalysis
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DOI：
10.1038/s43586-023-00207-0
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发表时间：
2023-04
期刊：
影响因子：
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通讯作者：
Shijie Deng;Brandon J Jolly;James R. Wilkes;Yu Mu;J. Byers;L. Do;Alexander J. M. Miller;Dunwei Wan
中科院分区：
文献类型：
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作者：
Shijie Deng;Brandon J Jolly;James R. Wilkes;Yu Mu;J. Byers;L. Do;Alexander J. M. Miller;Dunwei Wan
集成催化是一种新兴的方法，可以在一个反应容器中简化复杂产品的多步骤合成，实现高度控制，减少整个化学过程的浪费和成本。综合催化可以通过空间和时间控制来定义，以在一个锅中耦合不同的催化循环。这本初级读本讨论了常用的方法及其潜在的机制，并阐述了如何将空间和时间控制的催化集成在一个锅中可以高效地合成复杂的产品。重点介绍了集成催化的最新进展，分析了其应用现状和局限性，并对集成催化的未来发展进行了展望。
Integrated catalysis is an emerging methodology that can streamline the multi-step synthesis of complicated products in a single reaction vessel, achieving a high degree of control and reducing the waste and cost of an overall chemical process. Integrated catalysis can be defined using spatial and temporal control to couple different catalytic cycles in one pot. This Primer discusses commonly employed approaches and their underlying mechanisms and elaborates on how the integration of spatially and temporally controlled catalysis in one pot can deliver the synthesis of complex products with high efficiency. We highlight recent advances, analyse current applications and limitations, and provide an outlook for the future development of integrated catalysis.