Magnetic integrated metal/enzymatic nanoreactor for chemical warfare agent degradation
Magnetic integrated metal/enzymatic nanoreactor for chemical warfare agent degradation
复制标题
用于化学战剂降解的磁集成金属/酶纳米反应器
DOI：
10.1016/j.colsurfa.2019.03.061
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发表时间：
2019-06
期刊：
影响因子：
--
通讯作者：
Jiang Yanjun
中科院分区：
文献类型：
--
作者：
Li Haibin;Ma Li;Zhou Liya;Gao Jing;Huang Zhihong;He Ying;Jiang Yanjun
The combination of metal nanoparticle-catalysts and biocatalysts to perform cascade catalytic strategy is a powerful platform for synthesis or degradation of complex molecules. In this work, an integrated nanoreactor (INR) was successfully preparedviaimmobilizing organophosphorus hydrolase (OPH) onto porous carbon materials containing Co nanoparticles (C/Co). The C/Co was synthesized conveniently by pyrolysis of a metal-organic framework (MOF) named ZIF-67. This INR can reduce the toxicity of organophosphate nerve agent up to 208-fold by cascade degradation route. In this INR, C/Co not only acts as chemocatalyst but also serves as support for OPH, which allows an easy separation and reuse due to its magnetic properties. Moreover, this INR shows outstanding universal applicability, reusability and stability. With this proof-of-concept, it is foreseeable that the future metal nanoparticles that formed by pyrolyzing MOF will combine more other biocatalysts for perspective applications in more fields.
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DOI：
10.1016/j.colsurfa.2018.03.042
发表时间：
2018-06-20
影响因子：
5.2
作者：
Su, Shouzheng;Che, Rong;Wang, Jun
通讯作者：
Wang, Jun
影响因子：
3.7
作者：
Chun Wang;Haiyan Zhang;Cheng Feng;Shutao Gao;Ningzhao Shang;Zhi Wang
通讯作者：
Chun Wang;Haiyan Zhang;Cheng Feng;Shutao Gao;Ningzhao Shang;Zhi Wang
影响因子：
15.1
作者：
Gao, Jing;Kong, Weixi;Jiang, Yanjun
通讯作者：
Jiang, Yanjun
DOI：
10.1016/j.colsurfa.2018.01.042
发表时间：
2018-05-05
影响因子：
5.2
作者：
Yuan, Yi;Yang, Dan;Yan, Zhiming
通讯作者：
Yan, Zhiming
影响因子：
4.9
作者：
Jiangjiexing Wu;Sirong Li;Hui Wei
通讯作者：
Jiangjiexing Wu;Sirong Li;Hui Wei