Large enhancement of the nonlinear optical response of reduced fullerene derivatives
Large enhancement of the nonlinear optical response of reduced fullerene derivatives
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DOI：
10.1002/chem.200390175
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发表时间：
2003-04-04
影响因子：
4.3
通讯作者：
Prato, M
中科院分区：
文献类型：
--
作者：
Koudoumas, E;Konstantaki, M;Prato, M
研究了富勒吡咯烷及其盐及其还原形式的三阶非线性光学性质。减少后，响应会增加多达三个数量级，有时甚至超过三个数量级，给出的值与有史以来报告的最大值相当。计算和实验为这些新材料的非线性光学特性提供了相干图像。
The third-order nonlinear optical properties of fulleropyrrolidine, and its salt as well as their reduced forms are investigated. Upon reduction, the response increases by up to, and sometimes more than, three orders of magnitude, giving values comparable to the largest ever reported. Calculations and experiments provide a coherent picture for the nonlinear optical properties of these new materials.