A g-C3N4@Au@SrAl2O4:Eu2+,Dy3+ composite as an efficient plasmonic photocatalyst for round-the-clock environmental purification and hydrogen evolution
A g-C3N4@Au@SrAl2O4:Eu2+,Dy3+ composite as an efficient plasmonic photocatalyst for round-the-clock environmental purification and hydrogen evolution
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g-C3N4@Au@SrAl2O4:Eu2 ,Dy3 复合材料作为高效等离激元光催化剂,用于全天候环境净化和析氢
DOI:
10.1039/c9ta06423k
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发表时间:
2019-08-28
影响因子:
11.9
通讯作者:
Lin, Jun
中科院分区:
文献类型:
--
作者:
Liu, Xiaoming;Chen, Xueya;Lin, Jun
Here, we demonstrate a g-C3N4@Au@SrAl2O4:Eu2+,Dy3+ composite as a novel efficient self-luminous visible-light plasmonic photocatalyst for photocatalytic degradation of organic pollutants and hydrogen evolution from water around the clock. The g-C3N4@Au@SrAl2O4:Eu2+,Dy3+ composite was prepared by integrating a g-C3N4@Au plasmonic photocatalyst composite with a SrAl2O4:Eu2+,Dy3+ long-afterglow phosphor through a simple Pechini-type sol-gel method followed by a mechanical mixing and high-temperature calcination process. Owing to the synergistic effect of surface plasmon resonance of the Au nanoparticles in g-C3N4 and long-lasting phosphorescence of the SrAl2O4:Eu2+,Dy3+ phosphor, the prepared g-C3N4@Au@SrAl2O4:Eu2+,Dy3+ composite shows a continuous and efficient photocatalytic activity for photocatalytic degradation of organic pollutants and hydrogen evolution from water in a sunless environment. The current research study could provide a new strategy for designing a highly efficient composite photocatalyst for solar environmental purification and hydrogen energy production around the clock.