Picosecond laser-pump, x-ray probe spectroscopy of GaAs

Picosecond laser-pump, x-ray probe spectroscopy of GaAs
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GaAs 的皮秒激光泵浦、X 射线探针光谱

DOI:
10.1063/1.1516849
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发表时间:
2002
影响因子:
1.6
通讯作者:
D. Reis
D. Reis
中科院分区:
工程技术4区
文献类型:
--
作者:
B. Adams;M. DeCamp;E. Dufresne;D. Reis

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A laser-pump, x-ray probe spectroscopic experiment is described, and the results are shown. The Ga Kα x-ray fluorescence following x-ray absorption, at the Ga K absorption edge was measured, and its increase due to excitation with subpicosecond pulses of laser light at 4.6 eV photon energy was determined. The x-ray absorption, and thus the fluorescence, is increased for about 200 ps after the laser pulse because additional final states for the x-ray absorption are cleared in the valence band by the laser excitation. The technique could eventually lead to a femtosecond pump-probe spectroscopy with an absolute reference energy level and also to a femtosecond x-ray detector. This is of particular importance to future short-pulse x-ray sources, such as free-electron lasers.