Dual‐Atom Catalysts for Electrochemical Energy Technologies
Dual‐Atom Catalysts for Electrochemical Energy Technologies
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用于电化学能源技术的双原子催化剂
DOI：
10.1002/ente.202201456
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发表时间：
2023
影响因子：
3.8
通讯作者：
Chen, Shaowei
中科院分区：
文献类型：
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作者：
Cui, Tianchen;Liu, Qiming;Chen, Shaowei
高性能、低成本电催化剂的合理设计和工程是可持续能源技术发展的关键第一步。虽然单原子催化剂（SAC）已成为可行的候选者，但最近的研究表明，通过在附近引入第二个金属中心，形成双核构型，可以进一步操纵和增强其结构和活性。这种双原子催化剂（DAC）被认为是可行的选择，以打破SAC的局限性，由于双原子和它们的特殊结构之间的协同效应。本文综述了近年来DAC电催化剂在一系列重要反应中的合成、表征和性能研究进展。最后展望了未来的研究方向。
Rational design and engineering of high‐performance, low‐cost electrocatalysts represents a critical first step in the development of sustainable energy technologies. While single‐atom catalysts (SACs) have emerged as viable candidates, recent research has shown that the structure and activity can be further manipulated and enhanced by the incorporation of a second metal center in the close proximity, forming a binuclear configuration. Such dual‐atom catalysts (DACs) are recognized as feasible choices to break the limitations of SACs due to the synergetic effects between the bimetallic atoms and their special structures. Herein, the recent advances of DAC electrocatalysis for a range of important reactions, focusing on their synthesis, characterization, and performance, are summarized. The review is concluded with a perspective highlighting the challenges and future research directions.
用于电化学能量转换和存储的先进纳米材料
DOI：
--
发表时间：
2022
期刊：
影响因子：
--
作者：
Theodoros Daglis
通讯作者：
Theodoros Daglis