Research overview: The liquid-vapor interface of a metal as a vehicle for studying the atomic, electronic, and optical properties of an inhomogeneous liquid
Research overview: The liquid-vapor interface of a metal as a vehicle for studying the atomic, electronic, and optical properties of an inhomogeneous liquid
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研究概述：金属的液-气界面作为研究不均匀液体的原子、电子和光学特性的载体
DOI：
10.1073/pnas.84.14.4709
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发表时间：
1987
影响因子：
11.1
通讯作者：
S. Rice
中科院分区：
文献类型：
--
作者：
S. Rice
这份简短的报告旨在简要概述我对液体表面性质的研究。最后一句中的“液面”一词故意含糊其辞。当然，液-固、液-汽、液支撑单分子层界面的性质是不同的。我们也不应该期望原子、分子和金属液体与其他介质的几种界面是相同的。我将重点关注金属和合金的汽液界面的研究(简要介绍碳氢化合物单分子膜对支撑液态金属原子结构的影响)，因为它很好地说明了当现代理论和现代实验技术结合起来解决问题时可以取得的各种进展，而且因为所获得的一些结果与几年前的预期截然不同。
This short report is intended to give a brief overview of my research on the properties of the liquid surface. The phrase "liquid surface" in the last sentence is deliberately vague. Of course, the properties of the liquid-solid, the liquid-vapor, and the liquid-supported monolayer interfaces are not the same. Nor should we expect the several kinds of interfaces with other media of atomic, molecular, and metallic liquids to be the same. I will focus attention on the study of the liquid-vapor interface of metals and alloys (with a brief aside on the influence of a hydrocarbon monolayer on the atomic structure of the supporting liquid metal) because it illustrates nicely the kinds of advances that can be made when both modem theory and modern experimental technology are combined to solve problems, and because a number of the results obtained are very different from what was expected only a few years ago.