Method to establish the emission inventory of anthropogenic volatile organic compounds in China and its application in the period 2008-2012
Method to establish the emission inventory of anthropogenic volatile organic compounds in China and its application in the period 2008-2012
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DOI：
10.1016/j.atmosenv.2015.12.015
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发表时间：
2016-02-01
影响因子：
5
通讯作者：
Xie, Shaodong
中科院分区：
文献类型：
--
作者：
Wu, Rongrong;Bo, Yu;Xie, Shaodong
提出了一种建立中国VOC人为排放清单的方法，提出了4级源分类，建立了排放因子确定系统和参考数据库。并将其应用于建立2008-2012年期间的VOC排放清单。结果表明，中国人为VOC排放量从2008年的22.45 Tg增加到2012年的29.85 Tg，年均增长率为7.38%，山东、广东、江苏、浙江和河北是最大的排放省份。工业加工、运输和溶剂利用是主要来源，分别占2012年总排放量的39.3%、25.6%和14.9%。客车汽车、生物燃料燃烧、焦炭生产、生物质野外燃烧和原化学品制造是全国范围内的主要VOC来源。由于产业和能源结构不同，各省的主要来源也不同。中国挥发性有机化合物排放呈现出明显的空间差异，东部和东南部地区排放量远大于西北部，高排放区主要集中在环渤海经济圈、长江三角洲、珠江三角洲和四川盆地。2008-2012年期间，高排放区的规模扩大，污染严重的城市群逐渐出现。(C)2015爱思唯尔有限公司版权所有。
A method was developed to establish a comprehensive anthropogenic VOC emission inventory in China, in which a four-level source categorization was proposed, and an emission factor determination system together with a reference database were developed. And this was applied to establish VOC emission inventories for the period 2008-2012. Results show China's anthropogenic VOC emissions increased from 22.45 Tg in 2008 to 29.85 Tg in 2012 at an annual average rate of 7.38%, with Shandong, Guangdong, Jiangsu, Zhejiang and Hebei provinces being the largest emitters. Industrial processes, transportation and solvent utilization were the key sources, accounting for 39.3%, 25.6%, and 14.9% of the total emissions in 2012, respectively. Passenger cars, biofuel combustion, coke production, field burning of biomass, and raw chemical manufacturing were the primary VOC sources nationwide. The key sources for each province were different because of the disparate industry and energy structure. China's VOC emissions displayed remarkable spatial variation, with emissions in the east and southeast regions being much larger than in the northwest, and the high emission areas mainly centered in the Bohai Economic Rim, the Yangtze River Delta, the Pearl River Delta and the Sichuan Basin. The size of high emission areas expanded over the period 2008-2012, with heavily polluted city clusters gradually emerging. (C) 2015 Elsevier Ltd. All rights reserved.