CeFePO:: A heavy fermion metal with ferromagnetic correlations

CeFePO:: A heavy fermion metal with ferromagnetic correlations
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DOI:
10.1103/physrevlett.101.117206
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发表时间:
2008-09-12
影响因子:
8.6
通讯作者:
Geibel, C.
Geibel, C.
中科院分区:
物理与天体物理1区
文献类型:
--
作者:
Bruening, E. M.;Krellner, C.;Geibel, C.

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通过测量多晶的磁化率、比热、电阻率和核磁共振谱,研究了新型高温超导体RFePnO(1-x)F(x)的同系物CeFePO的基态性质。所有的结果表明,该化合物是一种磁无序的重费米子金属,近藤温度T(K)接近10 K,索末菲系数γ = 700 mJ/mol K(2),质量增强因子为50的数量级。磁化率数据和自旋弛豫时间的分析表明,强电子相关效应源于Ce-4f电子,而不是Fe-3d电子。增强的索默-威尔逊比R = 5.5以及Korringa乘积S(0)/T(1)TK(2)接近或等于0.065,远低于1,表明存在铁磁相关。因此,CeFePO似乎是在铁磁不稳定性的一侧。
The ground state properties of CeFePO, a homologue of the new high temperature superconductors RFePnO(1-x)F(x), were studied by means of susceptibility, specific heat, resistivity, and NMR measurements on polycrystals. All the results demonstrate that this compound is a magnetically nonordered heavy fermion metal with a Kondo temperature T(K) similar to 10 K, a Sommerfeld coefficient gamma = 700 mJ/mol K(2), and a mass enhancement factor of the order of 50. Analysis of the susceptibility data and of the spin relaxation time indicates that the strong electronic correlation effects originate from the Ce-4f electrons rather than from Fe-3d electrons. An enhanced Sommerfeld-Wilson ratio R = 5.5 as well as a Korringa product S(0)/T(1)TK(2) similar or equal to 0.065 well below 1 indicate the presence of ferromagnetic correlations. Therefore, CeFePO appears to be on the nonmagnetic side of a ferromagnetic instability.