Surface crystallization of amorphous solid water.
Surface crystallization of amorphous solid water.
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DOI：
10.1103/physrevlett.92.236101
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发表时间：
2004-06
影响因子：
8.6
通讯作者：
E. Backus;M. Grecea;A. Kleyn;M. Bonn
中科院分区：
文献类型：
--
作者：
E. Backus;M. Grecea;A. Kleyn;M. Bonn
我们证明了薄薄的无定形固体水层的晶化是在水面上开始的。这是通过观察无定形水在表面、本体和水-载体界面上的顺序结晶而得出的结论。表面形核模型定量地再现了观察到的三个位置的相变动力学。
We demonstrate that the crystallization of thin, supported amorphous solid water layers is initiated at the water surface. This is concluded from the observation of sequential crystallization of amorphous water at the surface, in the bulk, and at the water-support interface. A surface nucleation model quantitatively reproduces the observed transformation kinetics at the three sites.