Boson peak in manganites

Boson peak in manganites
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锰酸盐中的玻色子峰

DOI:
10.1088/1742-6596/486/1/012001
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发表时间:
2014
期刊:
Journal of Physics: Conference Series
影响因子:
--
通讯作者:
M.Dressel
M.Dressel
中科院分区:
--
文献类型:
--
作者:
B.P.Gorshunov;E.S.Zhukova;V.I.Torgashev;L.S. Kadyrov;E.A.Motovilova;F. Fischgrabe;V.Moshnyaga;T.Zhang;R.Kremer;U.Pracht;S.Zapf;M.Dressel

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在La1-xCaxMnO3(x≥0.5)相变为电荷有序介电相后,在TCO=2 40 K的相应温度以下,仅在x值相称的情况下,在太赫兹光谱范围内才出现一系列的吸收线.我们发现这些谱线起源于声学声子,这些声子通过布里渊区的折叠而变得光学活跃。在更低的温度下,在约20 cm−1-30 cm−1附近形成一个强烈不对称的额外吸收带,对应于约化布里渊区最低能量范霍夫奇点的位置。该能带被指定为玻色子峰值,即晶格振动态超过标准德拜贡献的部分。对于不相称的钙,折叠的声子和玻色子峰不会出现。
After the phase transition occurs in manganites La 1-x Ca x MnO 3 (x≥ 0.5) into a dielectric phase with charge order, right below the corresponding temperature of T CO= 240 K a series of absorption lines appear in the terahertz spectral range, only in case of commensurate x values. We show that the lines originate from acoustic phonons that become optically active by folding of the Brillouin zone. At even lower temperatures, a strongly asymmetric extra absorption band develops at frequencies around 20 cm− 1–30 cm− 1 corresponding to the position of the lowest-energy van Hove singularity in the reduced Brillouin zone. The band is assigned to the Boson Peak, ie to the excess of lattice vibrational states over the standard Debye contribution. The folded phonons and the boson peak do not show up for incommensurate calcium.
DOI: 10.1007/s10762-005-7600-y
发表时间: 2005-09-01
期刊: INTERNATIONAL JOURNAL OF INFRARED AND MILLIMETER WAVES
影响因子: --
作者:
Gorshunov, B;Volkov, A;Loidl, A
通讯作者: Loidl, A