Continuous selective conversion of methane to methanol over a Cu-KFI zeolite catalyst using a water–O2 mixture as the oxygen source
Continuous selective conversion of methane to methanol over a Cu-KFI zeolite catalyst using a water–O2 mixture as the oxygen source
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DOI：
10.1039/d3cc05379b
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发表时间：
2023
期刊：
影响因子：
--
通讯作者：
Yi Cao
中科院分区：
文献类型：
--
作者：
Hailong Zhang;Jiaxiu Guo;Yi Cao
The continuous catalytic oxidation of methane to methanol on a Cu-KFI zeolite using water–O2 mixture as the oxidant is reported. A high methanol space-time yield of 880.3 mmol molCu−1 h−1 with 83% selectivity is achieved at 450 °C. Isotopic labelling experiments show that both H2O and O2 provide the oxygen source in this catalytic methane-to-methanol conversion reaction.
