Magnetic ordering temperatures in rare earth metal dysprosium under ultrahigh pressures

Magnetic ordering temperatures in rare earth metal dysprosium under ultrahigh pressures
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超高压下稀土金属镝的磁有序温度

DOI:
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发表时间:
2014
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影响因子:
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通讯作者:
Y. Vohra
Y. Vohra
中科院分区:
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文献类型:
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作者:
G. Samudrala;G. Tsoi;S. Weir;Y. Vohra

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利用超灵敏电输运测量技术,研究了重稀土金属镝(Dy)在压力为69 GPa、温度为10 K条件下的磁有序温度。以往在高压下使用磁化率测量的研究只能在Dy的六方紧密堆积(hcp)相中追踪到7 GPa的磁有序温度。我们的研究表明,在hcp- sm相变中,磁有序温度突然下降80 K,然后逐渐下降,一直持续到17 GPa。随后,双hcp相的磁有序温度迅速升高,并最终在Dy的扭曲面中心立方相中趋于平稳。我们的研究重申,4f-壳仍然定位在Dy中,并且在高达69 GPa的压力下,没有磁矩损失或4f-壳离域。
Magnetic ordering temperatures in heavy rare earth metal dysprosium (Dy) have been studied using an ultrasensitive electrical transport measurement technique in a designer diamond anvil cell to a pressure of 69 GPa and a temperature of 10 K. Previous studies using magnetic susceptibility measurements at high pressures were able to track magnetic ordering temperature only till 7 GPa in the hexagonal close packed (hcp) phase of Dy. Our studies indicate that the magnetic ordering temperature shows an abrupt drop of 80 K at the hcp-Sm phase transition followed by a gradual decrease that continues till 17 GPa. This is followed by a rapid increase in the magnetic ordering temperatures in the double hcp phase and finally leveling off in the distorted face centered cubic phase of Dy. Our studies reaffirm that 4f-shell remains localized in Dy and there is no loss of magnetic moment or 4f-shell delocalization for pressures up to 69 GPa.