Plasma enhanced catalytic reforming of biomass tar model compound to syngas
Plasma enhanced catalytic reforming of biomass tar model compound to syngas
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DOI：
10.1016/j.fuel.2010.05.044
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发表时间：
2013-02-01
期刊：
影响因子：
7.4
通讯作者：
Tsubaki, Noritatsu
中科院分区：
文献类型：
--
作者：
Tao, Kai;Ohta, Naoko;Tsubaki, Noritatsu
以甲苯为模型化合物，对生物质焦油的直接热分解、等离子体辅助分解、催化蒸汽重整和等离子体强化催化蒸汽重整进行了比较研究。等离子体强化催化蒸汽重整效果最好。在催化重整反应中引入等离子体加速了甲苯的分解，而共存的Ni/SiO2重整催化剂则引导反应向CO和H-2的生成方向发展，实现了最高的甲苯转化率，同时也实现了最高的CO和H-2的生成速率。(C) 2010 Elsevier Ltd.版权所有。
Direct thermal decomposition, plasma-assisted decomposition, catalytic steam reforming and plasma enhanced catalytic steam reforming of biomass tar using toluene as a model compound were comparatively studied. Plasma enhanced catalytic steam reforming showed the best performance. The introduction of a plasma to the catalytic reforming reaction accelerated the decomposition of toluene, while the co-existing Ni/SiO2 reforming catalyst, on the other hand, guided the reaction towards formation of CO and H-2, realizing the highest toluene conversion, and the highest CO and H-2 formation rates simultaneously. (C) 2010 Elsevier Ltd. All rights reserved.