Sorption enhanced CO2 methanation
Sorption enhanced CO2 methanation
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DOI：
10.1039/c3cp51408k
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发表时间：
2013-01-01
影响因子：
3.3
通讯作者：
Zuettel, Andreas
中科院分区：
文献类型：
--
作者：
Borgschulte, Andreas;Gallandat, Noris;Zuettel, Andreas
从化石能源的盲目消费向可持续能源循环的转变最容易通过不改变基本的能源载体而是从可再生能源中产生来销售。碳氢化合物主要可以由生物质收集的可再生氢气和二氧化碳生产。然而，需要进行研究以提高该过程的能量和经济效率。我们证明了增强的CO2甲烷化的吸附增强催化。报道了以镍为载体的分子筛吸附催化剂的制备及其催化活性。吸附催化的功能进行了讨论，与确定的反应机理，提供新的途径在催化的影响。
The transformation from the fatuous consumption of fossil energy towards a sustainable energy circle is most easily marketable by not changing the underlying energy carrier but generating it from renewable energy. Hydrocarbons can be principally produced from renewable hydrogen and carbon dioxide collected by biomass. However, research is needed to increase the energetic and economic efficiency of the process. We demonstrate the enhancement of CO2 methanation by sorption enhanced catalysis. The preparation and catalytic activity of sorption catalysts based on Ni particles in zeolites is reported. The functioning of the sorption catalysis is discussed together with the determination of the reaction mechanism, providing implications for new ways in catalysis.