In situ and operando analysis of environmental catalysts - Studies on reaction mechanism and active site
In situ and operando analysis of environmental catalysts - Studies on reaction mechanism and active site
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环境催化剂的原位和操作分析-反应机理和活性位点研究
DOI：
10.1039/9781788016971-00242
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发表时间：
2019
期刊：
影响因子：
--
通讯作者：
A. Satsuma
中科院分区：
文献类型：
--
作者：
K. Murata;K. Ueda;Y. Mahara;J. Ohyama;A. Satsuma
原位分析和操作分析是观察反应条件下催化剂真实特征的方法。这些方法可以通过瞬态响应方法、动力学研究、催化剂和产物的温度依赖性等来阐明催化剂活性物种的动力学和催化剂表面的反应方案。这篇综述总结了原位和操作分析的进展，重点是环境催化剂，即燃烧催化剂、NO选择性还原、汽车三效催化和相关材料。
In situ and operando analyses are the methods to observe the real features of catalysts under the reaction conditions. These methods can clarify the dynamics of active species of catalysts and reaction scheme on catalyst surface through transient response method, kinetic study, temperature dependence of catalysts and products, and so on. In this review, progress in in situ and operando analyses is summarized with emphasis on environmental catalysts, ie, catalysts for combustion, selective reduction of NO, automotive three-way catalysis, and related materials.