Aromatics, reformulated gasoline, and atmospheric organic aerosol formation
Aromatics, reformulated gasoline, and atmospheric organic aerosol formation
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DOI：
10.1021/es960535l
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发表时间：
1997-07-01
影响因子：
11.4
通讯作者：
Seinfeld, JH
中科院分区：
文献类型：
--
作者：
Odum, JR;Jungkamp, TPW;Seinfeld, JH
二次有机气溶胶（SOA）的产率曲线已获得17个单独的芳香族物种从一个广泛的系列阳光照射烟雾室实验。这些产率曲线，解释的框架内的气体/气溶胶吸收模型，被用来定量占的SOA是在一系列的烟雾室实验中形成的12个不同的重新配制的汽油的整个蒸汽进行。由全部汽油蒸气的大气氧化产生的二次有机气溶胶的总量可以表示为燃料的各个芳族分子组分的贡献的总和。
Secondary organic aerosol (SOA) yield curves have been obtained for 17 individual aromatic species from an extensive series of sunlight-irradiated smog chamber experiments. These yield curves, interpreted within the framework of a gas/aerosol absorption model, are used to quantitatively account for the SOA that is formed in a series of smog chamber experiments performed with the whole vapor of 12 different reformulated gasolines. The total amount of secondary organic aerosol produced from the atmospheric oxidation of whole gasoline vapor can be represented as the sum of the contributions of the individual aromatic molecular constituents of the fuel.