Superionic states formation in group III oxides irradiated with ultrafast lasers.

Superionic states formation in group III oxides irradiated with ultrafast lasers.
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DOI:
10.1038/s41598-022-09681-0
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发表时间:
2022-04-05
期刊:
影响因子:
4.6
通讯作者:
Volkov AE
Volkov AE
中科院分区:
综合性期刊3区
文献类型:
--
作者:
Voronkov RA;Medvedev N;Volkov AE

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超快激光照射后,目标进入一个尚未探索的区域,其中固态物理与等离子体物理和化学重叠,产生了一种不寻常的协同作用--温暖的致密物质状态(WDM)。我们从理论上研究了具有高激发态电子系统的一些III族金属氧化物的WDM动力学和化学。我们采用密度泛函理论来研究在这些条件下材料非热跃迁到超离子态的可能性。在过渡期间分析材料的原子和电子性质,以深入了解指导这种转变的物理机制。
After ultrafast laser irradiation, a target enters a poorly explored regime where physics of a solid state overlaps with plasma physics and chemistry, creating an unusual synergy—a warm dense matter state (WDM). We study theoretically the WDM kinetics and chemistry in a number of group III-metal oxides with highly excited electronic system. We employ density functional theory to investigate a possibility of nonthermal transition of the materials into a superionic state under these conditions. Atomic and electronic properties of the materials are analyzed during the transitions to acquire insights into physical mechanisms guiding such transformations.
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