Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd3As2

Ultrahigh mobility and giant magnetoresistance in the Dirac semimetal Cd3As2
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DOI:
10.1038/nmat4143
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发表时间:
2015-03-01
期刊:
影响因子:
41.2
通讯作者:
Ong, N. P.
Ong, N. P.
中科院分区:
材料科学1区
文献类型:
--
作者:
Liang, Tian;Gibson, Quinn;Ong, N. P.

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狄拉克和外尔半金属是石墨烯的3D类似物,其中晶体对称性保护节点免受间隙形成(1-3)。Na 3Bi和Cd 3As 2被预测为狄拉克半金属(4,5),最近通过光电发射实验证实了这一点(6-8)。已经提出了狄拉克半金属在磁场中的几种新的输运性质(2,9 -11)。在这里,我们报告的性质Cd 3As 2是不可预测的,即一个显着的保护机制,强烈抑制反向散射在零磁场。在单晶中,保护导致在5 K下的载流子迁移率为9 × 10(6)cm(2)V-1 s(-1)。反向散射的抑制导致传输寿命比量子寿命长10(4)倍。通过施加的磁场解除这种保护导致非常大的磁阻。我们讨论了如何这可能涉及到费米面的变化所施加的磁场。
Dirac and Weyl semimetals are 3D analogues of graphene in which crystalline symmetry protects the nodes against gap formation(1-3). Na3Bi and Cd3As2 were predicted to be Dirac semimetals(4,5), and recently confirmed to be so by photoemission experiments(6-8). Several novel transport properties in a magnetic field have been proposed for Dirac semimetals(2,9-11). Here, we report a property of Cd3As2 that was unpredicted, namely a remarkable protection mechanism that strongly suppresses backscattering in zero magnetic field. In single crystals, the protection results in ultrahigh mobility, 9 x 10(6) cm(2) V-1 s(-1) at 5 K. Suppression of backscattering results in a transport lifetime 10(4) times longer than the quantum lifetime. The lifting of this protection by the applied magnetic field leads to a very large magnetoresistance. We discuss how this may relate to changes to the Fermi surface induced by the applied magnetic field.