Measuring the Dzyaloshinskii-Moriya interaction in a weak ferromagnet

Measuring the Dzyaloshinskii-Moriya interaction in a weak ferromagnet
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DOI:
10.1038/nphys2859
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发表时间:
2014-03-01
期刊:
影响因子:
19.6
通讯作者:
Katsnelson, M. I.
Katsnelson, M. I.
中科院分区:
物理与天体物理1区
文献类型:
--
作者:
Dmitrienko, V. E.;Ovchinnikova, E. N.;Katsnelson, M. I.

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磁性(材料中原子矩的自发排列)是由在原子间距离上运行的量子力学交换相互作用驱动的。一些磁相互作用会导致(1,2)原子排列的扭曲,或者由(3,4)引起。这可能导致磁电效应(预计将在未来技术中发挥重要作用)以及弱铁磁性现象(受所谓的 Dzyaloshinskii-Moriya 相互作用控制)(5-8)。在这里,我们通过使用同步辐射确定硼酸铁 (FeBO3) 中后者相互作用的符号。我们提出了一种基于两个 X 射线散射过程之间的干涉的新颖实验技术,其中一个作为参考波。我们的实验结果通过最先进的从头计算得到验证。我们的实验和理论方法有望共同为探索、建模和开发新型磁性和磁电材料开辟新的可能性。
Magnetism-the spontaneous alignment of atomic moments in a material-is driven by quantum mechanical exchange interactions that operate over interatomic distances. Some magnetic interactions cause(1,2), or are caused by(3,4), a twisting of arrangements of atoms. This can lead to the magnetoelectric effect, predicted to play a prominent role in future technology, and to the phenomenon of weak ferromagnetism, governed by the so-called Dzyaloshinskii-Moriya interaction(5-8). Here we determine the sign of the latter interaction in iron borate (FeBO3) by using synchrotron radiation. We present a novel experimental technique based on the interference between two X-ray scattering processes, where one acts as a reference wave. Our experimental results are validated by state-of-the-art ab initio calculations. Together, our experimental and theoretical approaches are expected to open up new possibilities for exploring, modelling and exploiting novel magnetic and magnetoelectric materials.