Detecting nuclear spins in an organosilane monolayer using nitrogen-vacancy centers for analysis of precursor self-assembly on diamond surface

Detecting nuclear spins in an organosilane monolayer using nitrogen-vacancy centers for analysis of precursor self-assembly on diamond surface
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DOI:
10.35848/1347-4065/accc91
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发表时间:
2023-05
影响因子:
1.5
通讯作者:
Y. Ueda;Yuto Miyake;Akirabha Chanuntranont;K. Otani;Masatomo Tsugawa;Daiki Saito;Shuntaro Usui;T. Teraji;S. Onoda;T. Shinada;H. Kawarada;T. Tanii
Y. Ueda;Yuto Miyake;Akirabha Chanuntranont;K. Otani;Masatomo Tsugawa;Daiki Saito;Shuntaro Usui;T. Teraji;S. Onoda;T. Shinada;H. Kawarada;T. Tanii
中科院分区:
物理与天体物理4区
文献类型:
--
作者:
Y. Ueda;Yuto Miyake;Akirabha Chanuntranont;K. Otani;Masatomo Tsugawa;Daiki Saito;Shuntaro Usui;T. Teraji;S. Onoda;T. Shinada;H. Kawarada;T. Tanii

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We demonstrated the correlation spectroscopy of organosilane monolayers using an ensemble of shallow nitrogen-vacancy centers as the quantum sensor. Several types of organosilane monolayers were grown directly on the diamond surface by exposing the surface to a silane precursor vapor. The feasibility of detecting 1H and 19F in the monolayer was examined by correlation spectroscopy measurements. The effect of the magnetic dipole–dipole interaction on the peak width was also discussed by comparing the spectrum of the monolayer with that of surface-attached 1H and that of immersion oil. The results highlight the feasibility of nitrogen-vacancy centers as the spin probe for physicochemical analyses of monolayers grown on the diamond surface.