Graphene/Organic Semiconductor Heterojunction Phototransistors with Broadband and Bi-directional Photoresponse
Graphene/Organic Semiconductor Heterojunction Phototransistors with Broadband and Bi-directional Photoresponse
复制标题
具有宽带和双向光响应的石墨烯/有机半导体异质结光电晶体管
DOI：
10.1002/adma.201804020
复制
发表时间：
2018-12-06
影响因子：
29.4
通讯作者：
Wang, Xinran
中科院分区：
文献类型：
--
作者：
Han, Jiayue;Wang, Jun;Wang, Xinran
A graphene-semiconductor heterojunction is very attractive for realizing highly sensitive phototransistors due to the strong absorption of the semiconductor layer and the fast charge transport in the graphene. However, the photoresponse is usually limited to a narrow spectral range determined by the bandgap of the semiconductor. Here, an organic heterojunction (C-60/pentacene) is incorporated on graphene to realize a broadband (405-1550 nm) phototransistor with a high gain of 5.2 x 10(5) and a response time down to 275 mu s. The visible and near-infrared parts of the photoresponsivity (9127 A W-1@650 nm and 1800 A W-1@808 nm) come from the absorption of the organic layer and the graphene, respectively. For the first time, a bi-directional (positive and negative) photoresponse is demonstrated at different wavelengths, due to the opposite charge transfer direction of the photoexcited carriers enforced by the unique band alignment. Such tunability will enable new functionalities such as largescale real-time optical image and infrared focal plane array detection in the future.
