Dynamic shear modulus of a semiflexible polymer network

Dynamic shear modulus of a semiflexible polymer network
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DOI:
10.1103/physreve.58.r1241
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发表时间:
1998-08-01
期刊:
影响因子:
2.4
通讯作者:
MacKintosh, FC
MacKintosh, FC
中科院分区:
物理与天体物理3区
文献类型:
--
作者:
Gittes, F;MacKintosh, FC

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我们构建了一个模型的动态剪切模量G(Ω)的纠缠或交联的网络的半柔性聚合物,可以占高频标度行为,G(Ω)类似于Ω(3/4),最近已经观察到的生物聚合物F-肌动蛋白的解决方案。我们认为,这种行为不应该是唯一的F-肌动蛋白,而是应该是一个明确的特点,一般的半柔性聚合物。我们还报告分子动力学模拟,支持单丝响应,这是我们的网络剪切模量模型的基础。
We construct a model for the dynamic shear modulus G(omega) of entangled or crosslinked networks of semiflexible polymer that can account for the high-frequency scaling behavior, G(omega) similar to omega(3/4), that has recently been observed in solutions of the biopolymer F-actin. As we argue, this behavior should not be unique to F-actin, but rather should be a clear characteristic of semiflexible polymers in,general. We also report molecular dynamics simulations that support the single filament response that is the basis of our model for the network shear modulus.