Superlyophilic Interfaces and Their Applications
Superlyophilic Interfaces and Their Applications
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超亲界面及其应用
DOI：
10.1002/adma.201703120
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发表时间：
2017-12
影响因子：
29.4
通讯作者：
Tian Ye
中科院分区：
文献类型：
--
作者：
Zhu Zhongpeng;Zheng Shuang;Peng Shan;Zhao Yong;Tian Ye
超亲液界面表示对不同液体显示出强亲和力的界面，包括超亲水性、超亲油性和超两亲性界面。当与这些界面接触时，水滴或油滴倾向于以接近0°的接触角完全扩散，呈现出多功能应用，包括自清洁、防雾、可控液体输送、液体分离等。受自然界的启发，科学家们在过去的几十年里开发了各种人工超亲液（SLPL）界面。就尺寸特征而言，人工SLPL界面可以分为四类：i）0 D颗粒，其吸附或催化性能可以通过超亲液性显著增强; ii）1D微/纳米纤维或纳米管/通道，其可以有效地转移SLPL界面的液体; iii）二维平面SLPL界面，不同的功能分子可以均匀地沉积在其上，形成光滑和光滑的膜;和iv）3D结构，可以通过单独构建0 D、1D或2D SLPL材料或直接制造随机SLPL框架来获得，并且始终可以用作功能涂层或块体材料。在这里，自然和人工SLPL接口的简要介绍，其次是一个简短的讨论之间的限制亲液性和疏液性，然后快照的方法来产生SLPL接口。具体重点放在最近的成就，从零到三个维度构建SLPL接口。随后，将介绍SLPL接口在商业领域的广泛应用。最后，对该领域的未来挑战进行了总结和展望。
Superlyophilic interfaces denote interfaces displaying strong affinity to diverse liquids, including superhydrophilic, superoleophilic, and superamphiphilic interfaces. When coming in contact with these interfaces, water or oil droplets tend to spread completely with contact angles close to 0°, presenting versatile applications including self‐cleaning, antifogging, controllable liquid transport, liquid separation, and so forth. Inspired by nature, scientists have developed various kinds of artificial superlyophilic (SLPL) interfaces in the past decades. In terms of dimensional characteristics, the artificial SLPL interfaces can be divided into four categories: i) 0D particles, whose dispersibility or catalytic performance can be notably enhanced by superlyophilicity; ii) 1D micro‐/nanofibers or nanotubes/channels, which can efficiently transfer liquids with SLPL interfaces; iii) 2D flat SLPL interfaces, on which different functional molecules can be deposited uniformly, forming ultrathin and smooth films; and iv) 3D structures, which can be obtained by either constructing 0D, 1D, or 2D SLPL materials separately or directly fabricating random SLPL frameworks, and can always be used as functional coatings or bulk materials. Here, natural and artificial SLPL interfaces are briefly introduced, followed by a short discussion of the limit between lyophilicity and lyophobicity, and then a snapshot of methods to generate SLPL interfaces is given. Specific focus is placed on recent achievements of constructing SLPL interfaces from zero to three dimensions. Following that, broad applications of SLPL interfaces in commercial areas will be introduced. Finally, a short summary and outlook for future challenges in this field is presented.
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