Electrically controlled metal–insulator transition process in VO2 thin films
Electrically controlled metal–insulator transition process in VO2 thin films
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DOI:
10.1088/0953-8984/24/3/035601
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发表时间:
2012-01
期刊:
影响因子:
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通讯作者:
Yong Zhao;J. Hao;Changhong Chen;Zhaoyang Fan
中科院分区:
文献类型:
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作者:
Yong Zhao;J. Hao;Changhong Chen;Zhaoyang Fan
We report the evolution process of VO2 thin films from the insulating phase to the metallic phase under current injection for the two-electrode-based thin-film devices. Based on electrical characterization and Raman microscopic detection, it was found that there exist two critical current densities, based on which the insulator-to-metal transition process can be divided into three stages. In stage I with low current injection, the VO2 film in the insulating (semiconducting) phase acts as a resistor until the first critical current density, above which the insulator–metal transition is a percolation process with metallic rutile and insulating monoclinic phases coexisting (stage II); while beyond a second critical current density, a filamentary current path with pure metallic phase is formed with the remaining part outside of the current path receding back to the pure insulating phase (stage III). We confirm that a critical current density is required for the onset of electrically induced insulator-to-metal transition in VO2 thin films.