Synthesis of Porous Hybrid Materials based on Layered Silicates: Functional Intercalates, Separation, and Catalysis (A06)

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An optimized melt synthesis of a charge homogenous hectorite allows for fundamental insights into the process of swelling and provides various ways for the functionalization of internal and external surfaces. A general procedure based on osmotic swelling of 1D-heterostructures makes double stacks and Janus-type platelets accessible. Intercalation of spacers (pillars, nanoparticles) creates micropores materials for gas separation and catalysis. This project explores the application of functionalized colloidal layered silicates derived from various methods of structuring.