Porous compartmentalized multi-catalytic electrospun membranes for reaction cascades in one-pot using ‘Wolf-Lamb’ catalysts (A12)

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Compartmentalized fibrous membranes and fiber morphologies with very high porosity and diverse pore size will be explored as novel multi-catalysts carrier for site-isolated immobilisation of incompatible (Wolf-Lamb type) catalysts in one-pot cascade reactions. The side-by-side and coaxial structures established in the first part of the project offer a unique opportunity for immobilisation of multiple catalysts in a site-specific manner with additional advantages of high porosity required for mass transport, upscalability and reusability. The study will combine experiments and computer simulations to make quantitative predictions and to understand the catalytic processes in flows through geometrically complex media.