Photoionization dynamics in chiral molecules: Understanding electron correlation and maximizing chiral response (C02)

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Photoionization experiments are a prime tool to investigate chirality of molecules in the gas phase. In this project we will develop a time-dependent ab initio description of such experiments, addressing the challeng-es of an adequate model for the chiral photoelectron continuum and a systematic treatment of electron cor-relation. Combining this approach with quantum control theory, we seek to determine the ultimate strength of chiral signals that can be obtained with randomly oriented molecules.