MAGNETIC STRUCTURE AND FIELD INDUCED PHASE TRANSITION IN La_<2-x>Sr_xCuO_4
MAGNETIC STRUCTURE AND FIELD INDUCED PHASE TRANSITION IN La_<2-x>Sr_xCuO_4
批准号:
09640416
负责人:
FUKASE Tetsuo
金额:
$2.37万
依托单位:
依托单位国家:
日本
项目类别:
Grant-in-Aid for Scientific Research (C)
财政年份:
1997
资助国家:
日本
项目状态:
已结题
起止时间:
1997 至 1998
中文摘要
La_<2-x>Sr_xCuO_4在x-1/8附近表现出T_c的局部极小值和磁有序。超导电性和磁序之间的关系引起了人们的强烈兴趣。本项目研究了La_ Sr_xCuO_4(x-1/8)体系的磁有序和场致自旋结构相变<2-x>。用弹性中子衍射方法测量了正交晶系La_ CuO_4的磁超晶格峰,<188>在四元数记法中,在倒数点(1/2* ε 1/2,0)和(1/2,1/2* ε 1,0)处观察到磁超晶格峰,表明它是一种调制的反铁磁有序,其不可逆性为ε-0.126,与Tranquada等人观察到的La_<1.48>Nd_<0.40>Sr_<0.12>CuO_4的情况相似。在低温四氢呋喃(TLT)相中。La_ Y_ySr_xCuO_4的La-NMR实验表明<2-x-y>,在正交晶系(OMT)相中,有序自旋的方向是沿着(0,*1 <minus-plus>delta*delta)_0,其中delta<<1,对于反铁磁La 关于我们 _<22-y>Y_yCuO_4和调制磁有序La_<2-x-y>Y_ySrxCuO_4(x-1/8),另一方面,在TLT相中,有序自旋的方向是沿着(*1,* 1,0)_0。当磁场沿着(0,1,0)_0方向施加时,在6-12 T的磁场下,发生从(0,1 *1 <minus-plus>delta,*delta)_0到(*1,<minus-plus>delta,0,0)_0的自旋翻转。在La_ Sr_ CuO_4的情况下<1.88><0.12>,OMT结构的不稳定性在低于15 K的低温下发光,观察到(*1,* 1,0)_0的自旋翻转,由于从OMT到ThT相的结构变化,观察到弹性异常。根据4.2 K下La-NMR共振峰宽的分析,估算了Cu-3d有序自旋的磁矩和磁有序态的体积百分比分别为μ<1.88>_<0.12><cu>(-0.32)μ_(B)和μ_(-100)%.测量了磁通线晶格的弹性常数,估计超导态的体积百分比大于90%,因此,在SrCuO_4晶体的几乎整个部分上,超导性与微观上的磁序共存<0.12>。与最佳掺杂样品(chi-0.15)相比,超导波动非常小,特别是在较低的温度下。少
英文摘要
La_<2-x>Sr_xCuO_4 shows local minimum of T_c and a magnetic ordering around x-1/8. The relation between superconductivity and the magnetic order is strongly interested. In this project the magnetic order and field induced phase transition of the spin structure was investigated in La_<2-x>Sr_xCuO_4(x-1/8). Magnetic superlattice peaks have been observed in elastic neutron-diffraction measurements on orthorhombic La_<188> CuO_4 at reciprocal points of (l/2*epsilon1/2,0), and (1/2,1/2*epsilon, 0), in the tetragonal notation, suggesting a modulated antiferromagnetic order with the incommensurability epsilon-0.126 similar to the case of La_<1.48>Nd_<0.40>Sr_<0.12>CuO_4 observed by Tranquada et. al. in the low-temperature tetragonal (TLT) phase. It is revealed from La-NMR experiments on La_<2-x-y>Y_ySr_xCuO_4 that the direction of the ordered spin in the orthorhombic (OMT) phase is along (0, *1<minus-plus>delta*delta)_0 in the orthorhombic notation where delta<<1 both for antiferromagnetic La … More _<22-y>Y_yCuO_4 and for modulated magnetic ordering La_<2-x-y>Y_ySrxCuO4(x-1/8), on the other hand, in the TLT phase the direction of the ordered spin is along (*1, *1,0)_0. When the magnetic field is applied along (0,1,0)_0 in the OMT phase, spin-flop from (0,1*1<minus-plus>delta, *delta)_0 to (*1, <minus-plus>delta, 0,0)_0 occurs at a field of 6-12 T.In the case of La_<1.88>Sr_<0.12>CuO_4 where the instability of the OMT structure glows at lower temperatures below 15 K, the spin-flop to (*1, *1,0)_0 is observed with an elastic anomaly due to the structural change from the OMT to the ThT phase. The magnetic moment of ordered Cu-3d spin and volume percentage of the magnetic ordered state is estimated from the analysis of the resonance peak width of La-NMR of La_<1.88>Sr_<0.12>CuO_4 at 4.2 K to be mu_<cu> -0.32 mu_B and -100%, respectively. Elastic constants of the flux-line lattice is also measured and volume percentage of the superconducting state is estimated to be larger than 90%, therefore, superconductivity coexists with the magnetic order microscopically over the almost whole part of the Sr_<0.12>CuO_4 crystal. The superconducting fluctuation reveals to be very small compared with an optimally doped sample (chi-0.15) especially at lower temperatures. Less
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T.Suzuki: "Observation of modulated magnetic long-range order in La_<2-x>Sr_xCuO_4." Phys.Rev.B. Vol.57, No.6. 3229-3232 (1998)
T.Suzuki:“La_<2-x>Sr_xCuO_4 中调制磁长程有序的观察。”
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T.Goto: "Field Induced Spin Reorientation and Low Temperature Structural Phase Transition in La_<2-x>Sr_xCuO_4" Physica B. Vol.246-247. 572-575 (1998)
T.Goto:“La_<2-x>Sr_xCuO_4 中的场诱导自旋重定向和低温结构相变”Physica B. Vol.246-247。
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T.Goto,: "^<139>La-NMR Study on La-based High-T_c Cuprates La_<2-x>M_xCuO_4(M=Sr, Ba)around x=0.115 under High Magnetic Field." J.Phys.Soc.Jpn.,. 66・9. 2870-2874 (1997)
T.Goto,:“强磁场下 x=0.115 附近 La 基高 T_c 铜酸盐 La_<2-x>M_xCuO_4(M=Sr, Ba) 的^<139>La-NMR 研究。”日本社会学会,66・9。
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T.Goto: "^<139>La-NMR Study on La-based High-T_c Cuprates La_<2-x>M_xCuO_4 (M=Sr, Ba) around x=0.115 under High Magnetic Field." J.Phys.Soc.Jpn.Vol.66, No.9. 2870-2874 (1997)
T.Goto:“高磁场下 x=0.115 附近 La 基高 T_c 铜酸盐 La_<2-x>M_xCuO_4 (M=Sr, Ba) 的 ^<139>La-NMR 研究”。
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T.Goto: "Field lnduced Spin Rcollentilljon and L.ow Tempcrature Suuctural Phase Tlansitron in L.a S_1 C_<AI>O_4" Physica B. 246-247. 572-575 (1998)
T.Goto:“L.a S_1 C_<AI>O_4 中的场诱导自旋 Rcollentilljon 和低温 Suuctural Phase Tlansitron”Physica B. 246-247。
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共 10 条
Development of liquid He free dilution refrigerator with Gifford-McMahon refrigerator.
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批准号:10554014
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项目类别:Grant-in-Aid for Scientific Research (B).
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资助金额:$8.26万
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财政年份:1998
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负责人:FUKASE Tetsuo
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依托单位: