Fabrication and study of magnetic competing systems in artificial superlattices

人工超晶格中磁竞争系统的制备和研究

• 批准号: 12640363
• 负责人: YAMAZAKI Hiroki
• 金额: $ 2.37万
• 依托单位: RIKEN (The Institute of Physical and Chemical Research)
• 依托单位国家: 日本
• 项目类别: Grant-in-Aid for Scientific Research (C)
• 财政年份: 2000
• 资助国家: 日本
• 起止时间: 2000 至 2002
• 项目状态: 已结题
• 来源: https://kaken.nii.ac.jp/grant/KAKENHI-PROJECT-12640363/
• 关键词: artificial lattice; magnetic anisotropy competition; exchange-coupling competition; heavy rare-earth metal; iron fluoride; neutron diffraction; frustration; ultra-thin film; 磁性人工格子; 超交換相互作用; 磁気異方性; 競合; 次元クロスオーバー; 絶縁体人工格子; 磁性競合系; 2次元磁性体; エピ

In this study, fabrication of the magnetic competing, with respect to magnetic antisotropy or exchange-coupling, systems was performed using artificial superlattices. Their magnetic properties were investigated in order to find out novel magnetic phases due to the magnetic competition. The magnetic systems with the competition in magnetic anisotropy were realized in the single-crystal Er/Tb superlattices grown parallel to the c-axis of hcp structure. Neutron diffraction study revealed that, as a function of temperature, the spin component parallel to the c-axis undergoes the same sequence including the Neel and Curie temperatures as bulk Er, while the component in the basal plane retains a helical ordering at higher temperatures up to 130K, which is more than twice the corresponding temperature of bulk Er. We argued that the basal-plane ferromagnetic ordering of the adjacent Tb layers enhanced the development of the basal-plane ordering in the Er layers. In order to study the magnetic systems with the competition in exchange-coupling, fluoride superlattices of FeF_2/ZnF_2 were prepared on single-crystal substrates. In addition to close structural characterization, dependence of the Neel temperature on the thickness of the FeF_2(001) and (110) ultra-thin layers was investigated. The observed periodic variations of the Neel temperature with a period of 1 atomic monolayer were discussed in terms of an interface-topographical frustration due to the competing exchange-coupling of J_2 and J_3. These superlattices can be regarded as "controlled competing systems" in contrast to the bulk dilute system of Fe_xZn_<1-x>F_2.

在这项研究中，制造的磁竞争，相对于磁各向异性或交换耦合，系统进行使用人工超晶格。研究了它们的磁性能，以发现由于磁竞争而产生的新磁相。在平行于hcp结构c轴生长的Er/Tb单晶超晶格中实现了磁各向异性竞争的磁性系统。中子衍射研究表明，作为温度的函数，平行于c轴的自旋分量经历与体Er相同的序列，包括Neel和居里温度，而基面中的分量在高达130 K的较高温度下保持螺旋有序，这是体Er相应温度的两倍多。我们认为，相邻的Tb层的基面铁磁有序增强了Er层的基面有序的发展。为了研究存在交换耦合竞争的磁性体系，在单晶衬底上制备了FeF_2/ZnF_2氟化物超晶格。除了密切的结构表征外，还研究了Neel温度与FeF_2（001）和（110）超薄层厚度的关系。用J_2和J_3的竞争交换耦合引起的界面形貌阻挫讨论了所观察到的周期为1原子单层的Neel温度的周期变化。与Fe_xZn_ F_2的体稀体系相比，这些超晶格可以看作是“受控竞争体系”<1-x>。

项目成果

H.Yamazaki, J.Satooka: "Two-dimensional magnetism realized in FeF_2/ZnF_2 multilayers with nanoscale thickness"RIKEN Review. No.38. 14-17 (2001)

H.Yamazaki、J.Satooka：“在纳米级厚度的 FeF_2/ZnF_2 多层中实现二维磁性”RIKEN Review。

H.Yamazaki, J.Satooka: "Structural and magnetic properties of FeF_2(001)/ZnF_2(001) and FeF_2(110)/ZnF_2(110) superlattice"Journal of Physics : Condensed Matter. (印刷中). (2003)

H.Yamazaki、J.Satooka：“FeF_2(001)/ZnF_2(001) 和 FeF_2(110)/ZnF_2(110) 超晶格的结构和磁性”物理学杂志：凝聚态物质（出版中）。

H. Yamazaki and J. Satooka: "Magnetic phase transition of FeF_2/ZnF_2 superlattices"Journal of Magnetism and Magnetic Materials. Vol.240. 442-444 (2002)

H. Yamazaki和J. Satooka：“FeF_2/ZnF_2超晶格的磁性相变”《磁性与磁性材料杂志》。

H.Yamazaki et al.: "Magnetic Structures of an Er/Tb Superlattice Studied by Neutorn Diffraction"physica status solidi. Vol.228, No.3. 741-750 (2001)

H.Yamazaki 等人：“通过中子衍射研究的 Er/Tb 超晶格的磁性结构”物理状态固体。

Hiroki Yamazaki 他: "Magnetic pliase transition of FeF_2/ZnF_2 superlattices"Journal of Magnetism and Magnetic Materials. (未定). (2002)

Hiroki Yamazaki 等人：“FeF_2/ZnF_2 超晶格的磁性平纹转变”《磁性与磁性材料杂志》(2002)。