Developmentofnewelectronicstructuretheoriesthroughaperspectiveoftheresonancestructure

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In this project, our new resonance theory formulated on the basis of the second-quantized, biorthogonal operator was systematically examined, and extended togeneralized theories. The computed resonance weights were virtually independent not onlyon the choice of the orbital-localization scheme but also on basis set. The method wasfurther improved to treat four-electron systems. Furthermore, computations and analysisof many organic compounds in solution phase were performed.