“YIG/金属”异质纳米薄膜自旋输运过程中多重物理机制纠缠的研究
批准号:
51501159
项目类别:
青年科学基金项目
资助金额:
22.0 万元
负责人:
卢玉明
依托单位:
学科分类:
金属功能材料
结题年份:
2018
批准年份:
2015
项目状态:
已结题
项目参与者:
李冠男、李鱼辉、曾道富、魏娟
中文摘要
“铁磁绝缘体YIG/金属”异质纳米薄膜的自旋输运过程,纯自旋流效应、磁近邻效应、界面Rashba自旋-轨道耦合效应多重物理机制纠缠不清且存在重大争议,具有丰富的物理内涵,是近年来新兴绝缘体自旋电子学领域的研究热点。本项目围绕“YIG/金属”异质结构薄膜,利用先进的热电、低噪音磁阻、电场调制等输运表征手段,全面系统研究金属材料的不同自旋-轨道耦合强度和电子结构等因素对“YIG/金属”中所呈现相关物理机制的影响与规律;掌握磁近邻效应、界面Rashba自旋-轨道耦合效应发生的基本条件、随薄膜厚度的变化特点及对纯自旋流效应的影响规律,力求定量区分多重物理机制的各自贡献大小,发展定量化自旋霍尔角、自旋扩散长度等自旋流关键参量值的方法;在深刻理解磁近邻效应、界面Rashba自旋-轨道耦合效应微观机理的基础上,积极探索拓展自旋相关的热电材料体系,提升优化重要的应用技术参数,推进自旋热电器件的实用化进程。
英文摘要
Pure spin current effect, magnetic proximity effect as well as interficial Rashba spin-orbit coupling effect have been tightly intertwined and greatly debated in the spin-dependent transport processes of "ferromagnetic insulator YIG/metal" heterostructure nanometer films,which exhibits abundant physical connotation and has become one of the hotspots for research in the rapidly developing insulator spintronics.In this proposal, we will take advantage of our state of the art thermoelectricity,low-noise magnetoresistance, electric-field modulation and other transport measurements to systematically characterize the spin-dependent transport properties of "YIG/metal" heterostructure nanometer films. We will firstly study the effect of the spin-orbit coupling, electronic structure and other factors on the emerging related physical mechanisms.Then, we will investigate the prerequisite for magnetic proximity effect and interfical Rashba spin-orbit coupling effect, find out the thickness-dependent features for magnetic proximity effect and interfical Rashba spin-orbit coupling effect, and confirm that how magnetic proximity effect and interfical Rashba spin-orbit coupling effect can influence pure spin current effect. We will also pursue to separate individual contribution from the magnetic proximity effect, interficial Rashba spin-orbit coupling effect and pure spin current effect, and try to search the methods to quantify the key parameters of spin current including spin Hall angle as well as spin diffusion length.On the basis of deep understanding of the microscopic mechanisms,we will actively explore spin-related thermoelectric material systems,promote the important parameters for application,and further advance the practical process of spin-related thermoelectric devices.
热电材料可以将废热回收转化为电再利用,对建设能量节约型、环境友好型社会意义重大。在本项目中,我们致力于利用真空气相沉积、球磨热压烧结、第一性原理计算等方法探索发现新型高性能的热电材料及理解所涉及的物理机制。在典型自旋相关热电材料“YIG/Pt”中,无论Pt是否因磁近邻效应发生自旋极化,其中自旋霍尔效应和(或)反常霍尔效应的主导电子偏转机制都是斜交散射,同时低温下会引入量子受限尺度下的弱局域化机制。在非自旋相关热电材料的开发中,合作发现了一种高性能的热电材料,即p型TaFeSb基半Heusler合金,热电转化效率高达~11.4%,在较宽温区内也能保持超高的品质因子~1。同时,我们扩展了课题研究范围,完成了BiFeO3基多铁陶瓷掺杂改性的前期实验积累,系统研究了Ho、Sm、Zr、BaTiO3掺杂对BiFeO3基陶瓷多铁性能的影响规律。
期刊论文列表
专著列表
科研奖励列表
会议论文列表
专利列表
Discovery of TaFeSb-based half-Heuslers with high thermoelectric performance
发现具有高热电性能的 TaFeSb 基半高斯勒材料
DOI:
10.1038/s41467-018-08223-5
发表时间:
2019-01
期刊:
Nature Communications
影响因子:
16.6
作者:
[Hangtian Zhu, Jun Mao, Yuwei Li, Jifeng Sun, Yumei Wang, Qing Zhu, Guannan Li, Qichen Song, Jiawei Zhou, Yuhao Fu, Ran He, Tian Tong, Zihang Liu, Wuyang Ren, Li You, Zhiming Wang, Jun Luo, Andrei Sotnikov, Jiming Bao, Kornelius Nielsch, Gang Chen, David J. Singh, Zhifeng Ren]
通讯作者:
Zhifeng Ren
DOI:
10.1142/s0217979218500716
发表时间:
2017-12
期刊:
International Journal of Modern Physics B
影响因子:
1.7
作者:
[Guannan Li;Zhiqian Chen;Yuming Lu;Meng Hu;Lina Jiao;Haoting Zhao]
通讯作者:
Guannan Li;Zhiqian Chen;Yuming Lu;Meng Hu;Lina Jiao;Haoting Zhao
DOI:
--
发表时间:
2019
期刊:
功能材料
影响因子:
--
作者:
[赵浩婷, 杨如霞, 卢玉明, 李冠男]
通讯作者:
李冠男
基于Cantor类熵变无序合金磁性薄膜反常/拓扑能斯特效应的微型热电发电机原型器件构筑
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批准号:--
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项目类别:省市级项目
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资助金额:0.0万元
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批准年份:2025
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负责人:卢玉明
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依托单位:
国内基金
海外基金