大气气溶胶干沉降对青岛近海水域几种微量金属的输入

批准号:
49976020
项目类别:
面上项目
资助金额:
17.0 万元
负责人:
李先国
依托单位:
学科分类:
D0602.海洋化学
结题年份:
2002
批准年份:
1999
项目状态:
已结题
项目参与者:
冯丽娟、郁纬军、于海、魏丽晖、江玉、薛秋红
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中文摘要
大气气溶胶干沉降是海洋中某些微量金属的重要外部来源,气溶胶的物理、化学性质对其沉降通量有很大影响。本研究以青岛近海水域为例,测定和了解气溶胶的主要物理、化学性质和控制因素;测定气溶胶干沉降向海洋输入微量金属的通量;从一个侧面了解大气气溶胶对近海水域生态环境的影响。这对海洋中微量金属循环和全球变化研究具有重大意义。
英文摘要
TSP and PM10 samples were simultaneously collected at three sites in Qingdao area. The concentrations of several trace metals in the samples were determined by means of ICP-AES. The deposition fluxes to the Qingdao coastal waters were estimated. The morphology of aerosol particles and the existing form of metals in the samples were systematically studied. A new parameterization method was put forward based on a modified dry deposition model. The results indicated that the concentrations of TSP, PM10 and trace metals were closely related to the functionality of the locality. Obvious temporal variation of the concentrations was observed. The relative concentrations of anthropogenic metals in PM10 were clearly higher than those in TSP. During floating dust or smog period in springtime, the concentrations of TSP, PM10 and crustal metals were pronouncedly elevated, with little changes in the concentrations of anthropogenic metals. Both direct determination and indirect estimation showed that the deposition fluxes of crustal elements to the Qingdao coastal waters in springtime accounted for more than 50 percent of the annual fluxes, while those in summertime accounted for less than 10 percent. On the other hand, the temporal variation of the fluxes for anthropogenic elements was much less. The iron in aerosol samples is mainly presented in the form of Fe2O3, with a small amount of FeO mixed together. The morphology of aerosol particles is very rich. The relationship between the morphology and the composition is very complicated.
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DOI:--
发表时间:--
期刊:海洋环境科学
影响因子:--
作者:陈兴茂;冯丽娟;张安慧;祁建华;张曼平;李先国
通讯作者:李先国
DOI:--
发表时间:--
期刊:中国海洋大学学报
影响因子:--
作者:祁建华;李培良;李先国;冯丽娟;张曼平
通讯作者:张曼平
Characterization of dust and non-dust aerosols with SEM/EDX
使用 SEM/EDX 表征粉尘和非粉尘气溶胶
DOI:10.1007/bf02919381
发表时间:2006
期刊:Journal of Ocean University of China
影响因子:1.6
作者:Q. Jianhua;Liu Xianguo;Feng Lijuan;Zhang Man
通讯作者:Zhang Man
DOI:10.1016/j.jaerosci.2005.04.005
发表时间:2006-02
期刊:Journal of Aerosol Science
影响因子:4.5
作者:J. Qi;Lijuan Feng;Xianguo Li;Manping Zhang
通讯作者:J. Qi;Lijuan Feng;Xianguo Li;Manping Zhang
DOI:--
发表时间:--
期刊:中国海洋大学学报
影响因子:--
作者:冯丽娟;李先国;祁建华;陈兴茂;张曼平
通讯作者:张曼平
植被与气候变化在我国渤、黄、东海陆架泥质区中的木质素分子化石和稳定同位素沉积记录
- 批准号:41276067
- 项目类别:面上项目
- 资助金额:84.0万元
- 批准年份:2012
- 负责人:李先国
- 依托单位:
利用多维稳定同位素分析研究天然表层水中烷基酚的光化学降解机理
- 批准号:40976041
- 项目类别:面上项目
- 资助金额:47.0万元
- 批准年份:2009
- 负责人:李先国
- 依托单位:
单体同位素分析与特征代谢产物分析联合用于近海沉积物中几种有机污染物的生物降解研究
- 批准号:20775074
- 项目类别:面上项目
- 资助金额:28.0万元
- 批准年份:2007
- 负责人:李先国
- 依托单位:
国内基金
海外基金
