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室温大能量宽调谐Fe:CdTe中红外激光技术研究

批准号:
62075221
项目类别:
面上项目
资助金额:
60.0 万元
负责人:
葛文琦
学科分类:
激光
结题年份:
2024
批准年份:
2020
项目状态:
已结题
项目参与者:
葛文琦

项目摘要

结项摘要

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中文摘要
5-7μm中红外激光在分子光谱学、呼出气体医学诊断和爆炸物稽查等领域有重要应用前景。长期以来,该波段激光的产生技术严重匮乏。Fe:CdTe晶体具有优良的物理特性和光谱特性,是实现大能量、宽调谐中红外激光输出最有前途的材料之一。由于Fe2+离子上能级寿命随温度升高迅速下降,室温Fe:CdTe激光器只能通过窄脉冲光源泵浦才能获得高效输出。受2.94μm窄脉冲激光泵浦源能量的限制,目前此类激光最高输出能量仅为2-3mJ。本项目以3.8μm非链式高能窄脉冲DF激光器泵浦Fe:CdTe晶体,通过有效抑制横向寄生振荡,获得高效激光输出。采用小角度双向对称泵浦方案和光栅谐振腔,可将室温Fe:CdTe激光脉冲能量提高数十倍,在室温条件下获得脉冲能量>100mJ、波长调谐范围>1μm的Fe:CdTe中红外激光输出。通过解决相关机理与技术问题,探索实现大能量、宽调谐室温中红外激光输出的新途径。
英文摘要
The mid-IR laser sources operating in the 5-7μm wavelength region are in great demand for a variety of applications including molecular spectroscopy, Breath analysis for non-invasive medical diagnostics, stand-off detection of explosion hazards. There is a lack of robust solid-state mid-IR laser sources with widely tunable output in this waveband. Fe:CdTe crystal offers a unique blend of physical (high thermal conductivity, low saturation intensity), spectroscopic characteristics(ultrabroad gain bandwidth, high absorption coefficient) that make it the gain media of choice for effective tunable lasing in the mid-IR region. Problem with this active material arises from the fact that the upper laser level lifetime of Fe2+ ions in CdTe sharply shortens with elevated temperature. To achieve satisfactory efficiencies at room temperature, it is necessary to excite the crystal by short pulses. The energy of Fe:CdTe laser in this case was only 2-3mJ, limited by the low energies of 2.94μm Q-switched solid-state lasers used for pumping. .In this project, the characteristics of Fe:CdTe laser in a scheme with two sides small angle pumping by a nonchain discharge pulsed high energy DF laser will be studied. Transversal parasitic oscillation must be suppressed for efficient lasing. The aim of the project is obtaining room temperature Fe:CdTe laser with output energy E>100mJ, widely tunable over the whole spectral range of 5.1-6.3μm with grating resonator. By solving the mechanical problems and key technologies, a novel routine for realizing room temperature high energy widely tunable Fe:CdTe laser will be explored.
5-7μm中红外激光在分子光谱学、呼出气体医学诊断和爆炸物稽查等领域有重要应用前景。长期以来,该波段激光的产生技术严重匮乏。Ⅱ~Ⅵ族晶体在中红外波段有一个较宽的透明波段,以掺杂Fe离子的Ⅱ~Ⅵ族晶体,作为增益介质的激光器件可实现中红外激光输出,并具有峰值功率高、脉宽窄、波长可调谐等优势。由于Fe2+离子上能级寿命随温度升高迅速下降,室温掺杂Fe晶体激光器只能通过窄脉冲光源泵浦才能获得高效输出。由于固体激光泵浦源受能量限制,本项目以3.8μm波长非链式高能窄脉冲DF激光器泵浦掺杂Fe晶体,获得高能量激光输出。项目组开展了国产Fe:CdSe等晶体的光谱特性研究。利用傅里叶中红外光谱仪对Fe:CdSe晶体的在2.5-5.5μm波段吸收光谱进行了测试;利用3μm波段中红外OPO激光器作为激发源,对Fe:CdSe晶体的吸收系数、发射光谱等开展了测试;得到了Fe:CdSe晶体的吸收截面积、发射截面积等关键参数。开展了非链式窄脉冲DF激光泵浦掺Fe晶体激光器的研究。建立掺Fe晶体激光的四能级速率方程。模拟了增益开关模式下,大能量窄脉冲DF激光泵浦泵浦掺Fe晶体激光器脉冲激光输出的物理过程和激光特性。在实验中搭建了非链式窄脉冲DF激光泵浦掺Fe晶体激光器。利用非链式窄脉冲DF激光泵浦,获得了中红外波长掺Fe晶体激光器的mJ级大能量脉冲输出。本项目的科学意义在于,通过表征国产Fe:CdSe晶体的关键参数,为生长性能优良的国产晶体提供基础实验数据;探索非链式高能窄脉冲DF激光作为泵浦源,在室温条件下实现脉冲掺Fe晶体的中红外激光输出。这将会填补5μm附近波段的室温高能量中红外激光器的空白,在生物医学、光电对抗和遥感探测等领域具有广阔的应用前景。
全固态自拉曼飞秒激光技术的研究
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