吸附剂的再生是吸附领域的瓶颈问题，如何在吸附剂上实现有机污染物高效吸附和完全降解是研究热点和难点。本研究拟研发可重复使用的纳米碳基复合吸附材料，能够高效吸附水中微量的典型药物和个人护理品（PPCPs），并在再生或吸附过程中氧化降解吸附的PPCPs，同时实现吸附剂的再生和污染物的降解。 主要内容包括研制可再生的具有介孔结构的颗粒碳纳米管和负载金属催化剂的复合石墨烯或碳纳米管吸附材料；研究该材料吸附典型PPCPs的特性和机制；利用纳米碳材料的高稳定性和导电性，研究通过低温加热、化学试剂氧化和电化学氧化等再生方式，完全氧化降解吸附在材料上的PPCPs，实现纳米吸附剂的再生和重复使用；构建基于负载催化剂的纳米碳基复合材料的吸附电化学降解装置，阐明PPCPs快速吸附同时被电化学氧化降解的特性和机制。本研究能拓展纳米碳材料在环境吸附领域的应用，为给水和污水处理中去除微量新兴污染物提供理论和技术支持。

Adsorbent regeneration is an important bottle-neck problem in adsorption area. It is hot and difficult to achieve the target for the adsorption and degradation of organic pollutants on the adsorbents. In this study, the regenerable nanocarbon-based hybrid adsorbents will be prepared to effectively adsorb some typical pharmaceutical and personal care products (PPCPs) from water and oxidize the adsorbed PPCPs in the adsorption or regeneration procsses, and both the adsorbent regeneration and the pollutant degradation can be achieved. The main researches include the preparation of regenerable granular carbon nanotubes with mesopores and metal catalyst-loaded graphene or carbon nanotubes,the adsorption behaviors and mechanism of PPCPs on these adsorbents, adsorbent regeneration and reuse as well as the complete oxidation and degradation of the PPCPs adsorbed on the adsorbents using the regeneration methods such as heating at low temperature,chemical reagent oxidation, and electrochemical oxidation due to the high stability and electroconductivity ofcarbon nanomaterials,the preparation of the adsorption and electrochemical oxidation setup based on the catalyst loaded carbon nanomaterials, and elucidation of the fast adsorption and electrochemical oxidation behavior and mechanism of PPCPs. This study will develop the application of carbon nanomaterials in the area of environmental area, and provide the theoretical and technical support for the removal of trace emerging contaminants in water and wastewater treatment.