High-Performance Flexible Photodetectors based on High-Quality Perovskite Thin Films by a Vapor-Solution Method

High-Performance Flexible Photodetectors based on High-Quality Perovskite Thin Films by a Vapor-Solution Method
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基于气相溶液法的高质量钙钛矿薄膜的高性能柔性光电探测器

DOI:
10.1002/adma.201703256
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发表时间:
2017-11-20
期刊:
影响因子:
29.4
通讯作者:
Pan, Anlian
Pan, Anlian
中科院分区:
材料科学1区
文献类型:
--
作者:
Hu, Wei;Huang, Wei;Pan, Anlian

文献摘要

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Organometal halide perovskites are new light-harvesting materials for lightweight and flexible optoelectronic devices due to their excellent optoelectronic properties and low-temperature process capability. However, the preparation of high-quality perovskite films on flexible substrates has still been a great challenge to date. Here, a novel vapor-solution method is developed to achieve uniform and pinhole-free organometal halide perovskite films on flexible indium tin oxide/poly(ethylene terephthalate) substrates. Based on the as-prepared high-quality perovskite thin films, high-performance flexible photodetectors (PDs) are constructed, which display a nR value of 81 A W-1 at a low working voltage of 1 V, three orders higher than that of previously reported flexible perovskite thin-film PDs. In addition, these flexible PDs exhibit excellent flexural stability and durability under various bending situations with their optoelectronic performance well retained. This breakthrough on the growth of high-quality perovskite thin films opens up a new avenue to develop high-performance flexible optoelectronic devices.