Palladium-catalyzed cascade oxidation/sp2 C-H acylation of azoarenes with aryl methanes.

Palladium-catalyzed cascade oxidation/sp2 C-H acylation of azoarenes with aryl methanes.
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DOI：
10.1021/ol402537t
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发表时间：
2013-10
期刊：
Organic letters
影响因子：
5.2
通讯作者：
Feng Xiong;C. Qian;Dongen Lin;W. Zeng;Xiaoxia Lu
Feng Xiong;C. Qian;Dongen Lin;W. Zeng;Xiaoxia Lu
中科院分区：
化学1区
文献类型：
--
作者：
Feng Xiong;C. Qian;Dongen Lin;W. Zeng;Xiaoxia Lu

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研究了钯催化偶氮芳烃的级联氧化/sp（2）C-H键酰化反应，以易得的芳基甲烷为原位生成的酰基源。该反应提供了在温和条件下方便地获得邻酰基偶氮芳烃的途径。
A Pd-catalyzed cascade oxidation/sp(2) C-H bond acylation of azoarenes was developed in which readily available aryl methanes were used as the in situ generated acyl sources. This reaction provides a convenient access to ortho-acyl azoarenes under mild conditions.