Pd9Ag1-N-doped-MOF-C: An efficient catalyst for catalytic transfer hydrogenation of nitro-compounds
Pd9Ag1-N-doped-MOF-C: An efficient catalyst for catalytic transfer hydrogenation of nitro-compounds
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Pd9Ag1-N-掺杂-MOF-C：硝基化合物催化转移氢化的高效催化剂
DOI：
10.1016/j.catcom.2017.02.019
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发表时间：
2017-05
影响因子：
3.7
通讯作者：
Zhi Wang
中科院分区：
文献类型：
--
作者：
Zong Liu;Wenhuan Dong;Saisai Cheng;Shuang Guo;Ningzhao Shang;Shutao Gao;Cheng Feng;Chun Wang;Zhi Wang
In this study,N-doped porous carbon (denoted asN-doped-MOF-C) was prepared by one-step carbonization of metal organic framework material, NH2-MIL-125. Pd and Ag nanoparticles were immobilized on theN-doped-MOF-C through co-reduction method with NaBH4as reductant. The results indicated that Pd9Ag1-N-doped-MOF-C catalyst exhibited excellent catalytic activity and selectivity for the catalytic transfer hydrogenation of nitroarenes using formic acid as the renewable hydrogen donor. The high catalytic activity of the catalyst can be attributed to the synergetic interaction between the support and the highly dispersed Pd and Ag metal nanoparticles.
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