Accurate measurements of CO2 mole fraction in the atmospheric surface layer by an affordable instrumentation

Accurate measurements of CO2 mole fraction in the atmospheric surface layer by an affordable instrumentation
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通过经济实惠的仪器准确测量大气表层中的二氧化碳摩尔分数

DOI:
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发表时间:
2014
期刊:
影响因子:
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通讯作者:
T. Vesala
T. Vesala
中科院分区:
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文献类型:
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作者:
P. Keronen;A. Reissell;F. Chevallier;E. Siivola;T. Pohja;V. Hiltunen;J. Hatakka;T. Aalto;L. Rivier;P. Ciais;A. Jordan;P. Hari;Y. Viisanen;T. Vesala

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We aimed to assess the feasibility of an affordable instrumentation, based on a non-dispersive infrared analyser, to obtain atmospheric CO2 mole fraction data for background CO2 measurements from a flux tower site in southern Finland. The measurement period was November 2006 to December 2011. We describe the instrumentation, calibration, measurements and data processing and a comparison between two analysers, inter-comparisons with a flask sampling system and with reference gas cylinders and a comparison with an independent inversion model. The obtained accuracy was better than 0.5 ppm. The inter-comparisons showed discrepancies ranging from -0.3 ppm to 0.06 ppm between the measured and reference data. The comparison between the analyzers showed a 0.1 +/- 0.4 ppm difference. The trend and phase of the measured and simulated data agreed generally well and the bias of the simulation was 0.2 +/- 3.3 ppm. The study highlighted the importance of quantifying all sources of measurement uncertainty.
DOI: 10.5194/essd-5-165-2013
发表时间: 2013-01-01
影响因子: 11.4
作者:
Le Quere, C.;Andres, R. J.;Zeng, N.
通讯作者: Zeng, N.