Optical emission spectroscopy of various materials irradiated by soft x-ray free-electron laser

Optical emission spectroscopy of various materials irradiated by soft x-ray free-electron laser
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软X射线自由电子激光照射下各种材料的发射光谱

DOI:
10.1117/12.822766
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发表时间:
2009
期刊:
--
影响因子:
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通讯作者:
Cihelka J
Cihelka J
中科院分区:
--
文献类型:
--
作者:
Cihelka J

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汉堡自由电子激光器(FLASH)输出的32.5nm和13.7nm的激光束分别被掠入射椭圆镜和离轴抛物面镜聚焦到20 μ m和1 μ m的光斑上。本文报道了能量为10 μJ的~10 fs脉冲在各种固体(Si,Al,Ti,Ta,Si_3N_4,BN,a-C/Si,Ni/Si,Cr/Si,Rh/Si,Ce:YAG,聚甲基丙烯酸甲酯- PMMA,不锈钢等)表面的掠入射和正入射聚焦。辐照度分别为1013 W/cm ~ 2和1016 W/cm ~ 2。在这些条件下产生的等离子体的光发射通过配备有iCCD头(iStar 720,Andor)的光栅(1200线/mm和/或150线/mm)光谱仪MS 257(Oriel)记录。令人惊讶的是,只有属于中性原子的线在1013 W/cm 2附近的强度下观察到。没有线的原子离子已被确定在紫外-可见光谱发射的等离子体形成的闪光灯光束聚焦在一个20微米的斑点。在1016 W/cm 2附近的强度下,OE光谱再次由原子线主导。然而,也记录到Al+和Al 2+的弱发射。Al/Al+的丰度比应至少为100。铝等离子体是非常冷的,通过计算机模拟铝等离子体OE谱,发现其激发温度为0.8eV。还记录了来自等离子体(典型的是碳;没有光谱线)和荧光体(在Ce:YAG晶体上,光谱仪记录了发光带和线等离子体发射)的宽带发射。
The beam of Free-Electron Laser in Hamburg (FLASH) tuned at either 32.5 nm or 13.7 nm was focused by a grazing incidence elliptical mirror and an off-axis parabolic mirror coated by Si/Mo multilayer on 20-micron and 1-micron spot, respectively. The grazing incidence and normal incidence focusing of ~10-fs pulses carrying an energy of 10 μJ lead at the surface of various solids (Si, Al, Ti, Ta, Si3N4, BN, a-C/Si, Ni/Si, Cr/Si, Rh/Si, Ce:YAG, poly(methyl methacrylate) - PMMA, stainless steel, etc.) to an irradiance of 1013W/cm2and 1016W/cm2, respectively. The optical emission of the plasmas produced under these conditions was registered by grating (1200 lines/mm and/or 150 lines/mm) spectrometer MS257 (Oriel) equipped with iCCD head (iStar 720, Andor). Surprisingly, only lines belonging to the neutral atoms were observed at intensities around 1013W/cm2. No lines of atomic ions have been identified in UV-vis spectra emitted from the plasmas formed by the FLASH beam focused in a 20-micron spot. At intensities around 1016W/cm2, the OE spectra are again dominated by the atomic lines. However, a weak emission of Al+and Al2+was registered as well. The abundance ratio of Al/Al+should be at least 100. The plasma is really cold, an excitation temperature equivalent to 0.8 eV was found by a computer simulation of the aluminum plasma OE spectrum. A broadband emission was also registered, both from the plasmas (typical is for carbon; there were no spectral lines) and the scintillators (on Ce:YAG crystal, both the luminescence bands and the line plasma emission were recorded by the spectrometer).
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发表时间: 1997
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DOI: 10.1117/12.822498
发表时间: 2009
期刊: Acta crystallographica. Section A, Foundations and advances
影响因子: --
作者:
S. Bajt;H. Chapman;A. Nelson;R. Lee;S. Toleikis;P. Mirkarimi;J. Alameda;S. Baker;H. Vollmer;R. Graff;A. Aquila;E. Gullikson;J. Meyer Ilse;E. Spiller;J. Krzywiński;L. Juha;J. Chalupský;V. Hájková;J. Hajdu;T. Tschentscher
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DOI: 10.1364/oe.15.006036
发表时间: 2007-05-14
期刊: OPTICS EXPRESS
影响因子: 3.8
作者:
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