Thickness Effects for Thermoelectric Property of Antimony Telluride Nanoplatelets via Solvothermal Method.
Thickness Effects for Thermoelectric Property of Antimony Telluride Nanoplatelets via Solvothermal Method.
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溶剂热法厚度对碲化锑纳米片热电性能的影响
DOI:
10.1038/srep37722
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发表时间:
2016-11-29
影响因子:
4.6
通讯作者:
Wang Z
中科院分区:
文献类型:
--
作者:
Yan X;Zheng W;Liu F;Yang S;Wang Z
Nanostructures have the potential to exhibit good thermoelectric properties by tuning and controlling their size and thickness, and the competing electrical and thermal properties can be decoupled by engineering the interface and grain boundary. In the present study, Sb2Te3nanoplatelets with different sizes were fabricated using a practical solvothermal method. The thickness of the platelets were regulated between sizes of 10 nm and 100 nm, and the opposite edge length was varied between 1 and 10 μm by altering chemical conditions. Consequently, manipulating the grain size made it suitable to benefit the carrier transport and also block phonons for the thin platelets, resulting in a significant decrease in thermal conductivity and simultaneous increase in electrical conductivity. The results showed that the optimized figure of meritZT, increased from 0.2 to 1.0 for thin samples, providing a comprehensive understanding of size-dependent thermoelectric performance.
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