Ex-CARS: exotic configuration for coherent anti-Stokes Raman scattering microspectroscopy utilizing two laser sources.

Ex-CARS: exotic configuration for coherent anti-Stokes Raman scattering microspectroscopy utilizing two laser sources.
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DOI:
10.1002/jbio.201000042
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发表时间:
2010-10
影响因子:
2.8
通讯作者:
Thomas, Robert
Thomas, Robert
中科院分区:
物理与天体物理2区
文献类型:
--
作者:
Yakovlev, Vladislav V.;Petrov, Georgi I.;Noojin, Gary D.;Harbert, Corey;Denton, Michael;Thomas, Robert

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我们提出并实验证明了一种新的相干反斯托克斯拉曼散射设置,它依赖于相干激发的拉曼振动使用宽带超短激光脉冲和信号读出使用传统的连续波激光辐射。这种特殊的布置不需要两个激光源的任何同步,并且可以用于非线性和自发拉曼信号的幅度的直接比较。时域(上图)和频域(下图)中的Ex-CARS。
We propose and experimentally demonstrate a new coherent anti-Stokes Raman scattering setting, which relies on a coherent excitation of Raman vibration using a broadband ultrashort laser pulse and signal read-out using a conventional continuous wave laser radiation. Such an exotic arrangement does not require any synchronization of two laser sources and can be used for direct comparison of amplitudes of nonlinear and spontaneous Raman signals. Ex-CARS in time- (top panel) and frequency- (bottom panel) domain.
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