The evolution of molecular machines through interfacial nanoarchitectonics: from toys to tools.
The evolution of molecular machines through interfacial nanoarchitectonics: from toys to tools.
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DOI：
10.1039/d0sc03164j
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发表时间：
2020-07-08
期刊：
影响因子：
8.4
通讯作者：
Ariga K
中科院分区：
文献类型：
--
作者：
Ariga K
分子机器通常被视为分子艺术品，有时被视为花哨的分子玩具。然而，许多研究人员努力将分子机器作为现实实际应用的有用工具。本文从分子机器从科学玩具到有用工具的演变角度，讨论了将分子机器的工作环境从溶液转变为界面介质的问题。在简要介绍了溶液中分子机器的传统研究及其在清洁固体表面上的纳米技术操纵之后，讨论了在动态界面(如液体表面)上分子机器操作的开创性研究，以及活细胞中分子机器功能及其模型的前沿研究。生物体内的生物分子机器是数十亿年进化的产物。我们可以用人工分子机器在短得多的时间内纳米构建这样复杂的功能系统。通过界面纳米结构，分子机器可以变得更加有用。
Molecular machines are often regarded as molecular artworks and sometimes as fancy molecular toys. However, many researchers strive to operate molecular machines as useful tools for realistic practical applications. In this perspective article, shifting the working environment of molecular machines from solution to interfacial media is discussed from the viewpoint of their evolution from scientific toys to useful tools. Following a short description of traditional research into molecular machines in solution and their nanotechnological manipulation on clean solid surfaces, pioneering research into molecular machine operation at dynamic interfaces, such as liquid surfaces, is discussed, along with cutting-edge research into molecular machine functions in living cells and their models. Biomolecular machines within organisms are the products of evolution over billions of years. We may nanoarchitect such sophisticated functional systems with artificial molecular machines within much shorter periods. Molecular machines can be made more useful with interfacial nanoarchitectonics.
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