Femtosecond X-ray-induced fragmentation of fullerenes

Femtosecond X-ray-induced fragmentation of fullerenes
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飞秒 X 射线诱导富勒烯碎裂

DOI:
10.1080/09500340.2015.1064175
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发表时间:
2015
影响因子:
1.3
通讯作者:
Berrah N
Berrah N
中科院分区:
物理与天体物理4区
文献类型:
--
作者:
Berrah N

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自由电子激光器是一种新型的飞秒、强、短波长激光器,它为研究许多科学领域的结构和动力学提供了新的机会。这些性能不断提高的新激光器使人们能够理解原子空间尺度和原子运动时间尺度上的物理和化学变化,这对广泛的科学领域至关重要。我们在这里描述的相互作用的富勒烯在多光子制度与直线加速器相干光源(LCLS)的X射线自由电子激光在SLAC国家实验室。特别是,我们报告的新数据,关于Ho3N@C80分子的电离,并与我们以前的C60调查的LCLS脉冲引起的辐射损伤的结果进行比较。我们还简要地讨论了新的可用的仪器,物理和化学科学的潜在影响时,他们加上自由电子激光以及理论计算和建模。
A new class of femtosecond, intense, short – wavelength lasers – the free-electron laser – has opened up new opportunities to investigate the structure and dynamics in many scientific areas. These new lasers, whose performance keeps increasing, enable the understanding of physical and chemical changes at an atomic spatial scale and on the time scale of atomic motion which is essential for a broad range of scientific fields. We describe here the interaction of fullerenes in the multiphoton regime with the Linac Coherent Light Source (LCLS) X-ray free-electron laser at SLAC National Laboratory. In particular, we report on new data regarding the ionization of Ho3N@C80molecules and compare the results with our prior C60investigation of radiation damage induced by the LCLS pulses. We also discuss briefly the potential impact of newly available instrumentation to physical and chemical sciences when they are coupled with FELs as well as theoretical calculations and modeling.
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