Electrochemical sensors and biosensors.

Electrochemical sensors and biosensors.
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DOI:
10.1021/ac202878q
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发表时间:
2012-01-17
影响因子:
7.4
通讯作者:
Cliffel, David E.
Cliffel, David E.
中科院分区:
化学1区
文献类型:
--
作者:
Kimmel, Danielle W.;LeBlanc, Gabriel;Meschievitz, Mika E.;Cliffel, David E.

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本文综述了2010年和2011年电化学和生物化学传感器的开发和应用进展。在选择学术文章,以促进这一审查,特别强调的是放在工作领域发表的参考电极,电位传感器,伏安传感器,电流传感器,生物传感器,免疫传感器和质量传感器。在过去的2年里,有一些重要的文件不属于较大部分中的一般小节。这些新的进展对于电化学传感器领域非常重要,因为它们为未来的研究开辟了新的途径和方法。上面的每一节都包含一个标题为“其他感兴趣的论文”的小节,其中包括这些文章,并描述了它们对该领域的重要性。例如,虽然用于感测感兴趣的分析物的大多数电化学技术是基于电势或电流的变化,但Shan等人1已经开发了一种用于执行电化学测量的全新方法。在他们的工作中,他们报告了一种使用表面等离子体共振(SPR)产生的电极表面的光学信号来成像局部电化学电流的方法。电化学电流图像是基于这样的事实,即电流密度可以很容易地从局部SPR信号计算。作者通过对金基底上指纹上的TNT痕迹进行成像来证明这一概念。全文和综述主要通过搜索ScienceScholar和ISI Web of Knowledge收集。通过替代数据库或通过细读相关出版物的分析期刊发现了其他文章。由于参考文献的限制,仅考虑纳入英文出版物。显然,已经有更多的出版帐户的开创性工作与电化学和生物化学传感器比这里所涵盖的。这篇综述是对现有文献的一个小样本,并不打算涵盖过去两年的每一个进展。所选文献侧重于新型传感器的材料、技术和临床相关应用的新趋势。确保适当的覆盖面
This review covers advances in electrochemical and biochem-ical sensor development and usage during 2010 and 2011. In choosing scholarly articles to contribute to this review, special emphasis was placed on work published in the areas of reference electrodes, potentiometric sensors, voltammetric sensors, amperometric sensors, biosensors, immunosensors, and mass sensors. In the past 2 years there have been a number of important papers that do not fall into the general subsections contained within the larger sections. Such novel advances are very important for the field of electrochemical sensors as they open up new avenues and methods for future research. Each section above contains a subsection titled “Other Papers of Interest” that includes such articles and describes their importance to the field in general. For example, while most electrochemical techniques for sensing analytes of interest are based on the changes in potential or current, Shan et al. 1 have developed a completely novel method for performing electrochemical measurements. In their work, they report a method for imaging local electrochemical current using the optical signal of the electrode surface generated from a surface plasmon resonance (SPR). The electrochemical current image is based on the fact that the current density can be easily calculated from the local SPR signal. The authors demonstrated this concept by imaging traces of TNT on a fingerprint on a gold substrate. Full articles and reviews were primarily amassed by searching the SciFinder Scholar and ISI Web of Knowledge. Additional articles were found through alternate databases or by perusing analytical journals for pertinent publications. Because of the reference limitation, only publications written in English were considered for inclusion. Obviously, there have been more published accounts of groundbreaking work with electrochemical and biochemical sensors than those covered here. This review is a small sampling of the available literature and not intended to cover every advance of the past 2 years. The literature chosen focuses on new trends in materials, techniques, and clinically relevant applications of novel sensors. To ensure proper coverage
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