CAREER: Probing Antiferromagnetic Spintronics with Nitrogen-Vacancy Centers in Diamond

职业：利用金刚石中的氮空位中心探测反铁磁自旋电子学

• 批准号: 2046227
• 负责人: Chunhui Du
• 金额: $ 60.98万
• 依托单位: University of California-San Diego
• 依托单位国家: 美国
• 项目类别: Continuing Grant
• 财政年份: 2021
• 资助国家: 美国
• 起止时间: 2021-04-01 至 2023-09-30
• 项目状态: 已结题
• 来源: https://www.nsf.gov/awardsearch/showAward?AWD_ID=2046227&HistoricalAwards=false
• 关键词: CAREER; Probing; Antiferromagnetic; Spintronics; Nitrogen

Non-Technical Abstract:Antiferromagnets are advanced materials that are scientifically intriguing and technologically important. They have promising properties to bring new functionalities for developing next-generation information technologies, such as high-densities, ultrafast data processing speeds. Despite their potential benefits, these materials are difficult to investigate using conventional techniques. In this CAREER project, the principal investigator introduces nitrogen vacancy centers in diamond to achieve nanoscale quantum sensing and imaging of antiferromagnetic insulators. This technique provides a new perspective to reveal emergent antiferromagnetic spin transport and dynamic behaviors. This research project is integrated with education and outreach plan that promotes the participation of underrepresented minority students into science and technology careers as well as public access to some of the most exciting developments at the forefront of materials science research.Technical Abstract:Antiferromagnetic materials with exchange-enhanced magnon band gaps and vanishing net magnetization exhibit a wide range of exotic, unintuitive, and technically interesting phenomena. Examples include topologically protected magnetic textures, long-range spin transport, ultrafast magnetic switching, magnon Bose-Einstein condensation, and many others. Successful application of antiferromagnetic materials to functional spintronic devices requires a comprehensive understanding of these emergent material properties, which remains challenging in the current state-of-the-art. Here, the principal investigator employs nitrogen vacancy centers, optically active atomic spin defects in diamond, to perform quantum sensing and imaging of the local spin behaviors of antiferromagnetic insulators at the nanometer length scale. Exploiting the unprecedented field sensitivity and spatial resolution of nitrogen vacancy centers, the research team aims to reveal the fundamental mechanisms governing the intrinsic spin diffusion and Néel order switching in antiferromagnets. Taking advantage of the dipole-dipole interaction between antiferromagnetic magnons and nitrogen vacancy centers, the “stretch” goal of this project is to develop antiferromagnet-based hybrid systems for next-generation quantum information technologies. The proposed research is expected to make important contributions to the burgeoning field of “antiferromagnetic spintronics”. By developing cutting-edge quantum sensing and imaging techniques and demonstrating their operation in an ambient environment, the project provides a versatile measurement platform which can extend naturally to many other interesting magnetic systems and benefits the community in the long run by influencing future quantum sensing technologies.This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

非技术摘要：反铁磁体是一种先进材料，在科学上很有趣，在技术上也很重要。它们具有为开发下一代信息技术带来新功能的前景，例如高密度，超快的数据处理速度。尽管它们具有潜在的好处，但这些材料很难使用传统技术进行研究。在这个CAREER项目中，主要研究者在金刚石中引入氮空位中心，以实现反铁磁绝缘体的纳米级量子传感和成像。该技术为揭示突现反铁磁自旋输运和动力学行为提供了新的视角。这个研究项目是整合教育和推广计划，促进少数民族学生参与到科学和技术的职业生涯，以及公众获得一些最令人兴奋的发展，在材料科学研究的前沿。技术摘要：反铁磁材料与交换增强磁振子带隙和消失的净磁化表现出广泛的异国情调，不直观的，技术上有趣的现象。例子包括拓扑保护的磁性纹理，长程自旋输运，超快磁开关，磁振子玻色-爱因斯坦凝聚，和许多其他的。反铁磁材料的功能自旋电子器件的成功应用需要全面了解这些新兴的材料特性，这仍然是具有挑战性的，在目前的国家的最先进的。在这里，主要研究人员采用氮空位中心，光学活性原子自旋缺陷的金刚石，进行量子传感和成像的反铁磁绝缘体的局部自旋行为在纳米长度尺度。利用氮空位中心前所未有的场灵敏度和空间分辨率，研究小组旨在揭示反铁磁体中内在自旋扩散和Néel顺序切换的基本机制。利用反铁磁磁振子和氮空位中心之间的偶极-偶极相互作用，该项目的“延伸”目标是为下一代量子信息技术开发基于反铁磁的混合系统。该研究有望为新兴的“反铁磁自旋电子学”领域做出重要贡献。通过开发尖端的量子传感和成像技术，并展示它们在周围环境中的操作，该项目提供了一个多功能的测量平台，可以自然地扩展到许多其他有趣的磁系统，并通过影响未来的量子传感技术使社区长期受益。该奖项反映了NSF的法定使命，并通过使用基金会的知识价值和更广泛的影响审查标准。

项目成果

Quantum sensing and imaging of spin‐orbit‐torque‐driven spin dynamics in noncollinear antiferromagnet Mn 3 Sn

非共线反铁磁体 Mn 3 Sn 中自旋轨道扭矩驱动的自旋动力学的量子传感和成像

• DOI: 10.1002/adma.202200327
• 发表时间: 2022
• 期刊: Advanced Materials
• 影响因子: 29.4
• 作者: Yan, Gerald Q.;Li, Senlei;Lu, Hanyi;Huang, Mengqi;Xiao, Yuxuan;Wernert, Luke;Brock, Jeffrey A.;Fullerton, Eric E.;Chen, Hua;Wang, Hailong
• 通讯作者: Wang, Hailong

Quantum Imaging of Magnetic Phase Transitions and Spin Fluctuations in Intrinsic Magnetic Topological Nanoflakes

• DOI: 10.1021/acs.nanolett.2c01390
• 发表时间: 2022-07-11
• 期刊: NANO LETTERS
• 影响因子: 10.8
• 作者: McLaughlin, Nathan J.;Hu, Chaowei;Du, Chunhui Rita
• 通讯作者: Du, Chunhui Rita

Strong Correlation Between Superconductivity and Ferromagnetism in an Fe-Chalcogenide Superconductor

• DOI: 10.1021/acs.nanolett.1c02424
• 发表时间: 2021-08-20
• 期刊: NANO LETTERS
• 影响因子: 10.8
• 作者: McLaughlin, Nathan J.;Wang, Hailong;Du, Chunhui Rita
• 通讯作者: Du, Chunhui Rita

Electric-Field-Induced Coherent Control of Nitrogen-Vacancy Centers

氮空位中心的电场诱导相干控制

• DOI: 10.1103/physrevapplied.18.064031
• 发表时间: 2022
• 期刊: Physical Review Applied
• 影响因子: 4.6
• 作者: Yan, Gerald Q.;Li, Senlei;Yamamoto, Tatsuya;Huang, Mengqi;Mclaughlin, Nathan J.;Nozaki, Takayuki;Wang, Hailong;Yuasa, Shinji;Du, Chunhui Rita
• 通讯作者: Du, Chunhui Rita

Quantum sensing of local stray field environment of micron-scale magnetic disks

• DOI: 10.1063/5.0150709
• 发表时间: 2023-07
• 期刊: Applied Physics Letters
• 影响因子: 4
• 作者: Jin-Jian Zhou;Gerald Q. Yan;Mengqi Huang;N. McLaughlin;C. Du;Hailong Wang