CAREER: Exploring Nonlinear Electrodynamics from Topology and Correlation in Layered Quantum Materials

职业：从层状量子材料的拓扑和相关性探索非线性电动力学

• 批准号: 2143426
• 负责人: Qiong Ma
• 金额: $ 63.17万
• 依托单位: Boston College
• 依托单位国家: 美国
• 项目类别: Continuing Grant
• 财政年份: 2022
• 资助国家: 美国
• 起止时间: 2022-06-01 至 2027-05-31
• 项目状态: 未结题
• 来源: https://www.nsf.gov/awardsearch/showAward?AWD_ID=2143426&HistoricalAwards=false
• 关键词: CAREER; Exploring; Nonlinear; Electrodynamics; Topology

This award is funded in whole or in part under the American Rescue Plan Act of 2021 (Public Law 117-2). Nontechnical Description: How a material responds to electric and magnetic fields determines its functionality and its usefulness in electronic and optical devices. Nonlinear processes allow for interesting phenomena with widespread applications. For example, an optical limiting material can be transparent at low light intensity but opaque at high (and potentially hazardous) intensity. This allows a user to see under normal conditions while protecting them from injury. Nonlinear electromagnetic materials can address growing demands for devices with new functionality and higher efficiency. This CAREER project aims to explore new forms of nonlinear electromagnetism that arise from the quantum properties of electrons in novel two-dimensional quantum materials. The low dimensionality gives rise to new quantum confinement effects that can enable highly efficient and tunable electronic devices for information and energy technologies. The PI will explore the physics of atomically-thin layered quantum materials by fabricating ultrathin electronic devices from layered 2D materials and studying their nonlinear electromagnetic response at low temperatures. The project intimately integrates research activities, student mentoring, educational plans, and outreach initiatives centered around quantum materials, physics, and technology. The principal investigator is particularly dedicated to addressing gender inequality in physics by promoting female researchers and cultivating a young and vigorous force reserve through initiative programs. This project is jointly funded by the Electronic and Photonic Materials (EPM) and the Condensed Matter Physics (CMP) programs of the Division of Materials Research (DMR).Technical Description: Nonlinear electromagnetic responses are the phenomena where materials respond nonlinearly to external electromagnetic fields. Recent advances uncovered deep connections between nonlinear electromagnetic responses and topological and Berry curvature properties of quantum matter, leading to an emerging field of topological nonlinear electromagnetism. In this nascent field many questions need to be addressed. For instance, what are the signature nonlinear responses of new topological states and how large can they be? What is the role of impurities and scattering in those processes? What is the role of Coulomb interactions? Can we use those responses to probe and manipulate emergent phases? This CAREER project aims to answer those questions by exploring the physics in atomically-thin layered quantum materials with controllable Fermi energy, band structures, symmetry, topology and electron interactions through electrostatic gating, van der Waals stacking and layer twisting. The investigator develops innovative fabrication methods to create ultrathin electronic devices from those materials and investigates their nonlinear electromagnetic properties in a home-built multi-functional magneto-transport/optics cryo-system with broadband electromagnetic excitation. Combining highly-tunable nonlinear materials with broadband excitation will permit exploration of previously inaccessible regimes in topological and correlated materials.This award reflects NSF's statutory mission and has been deemed worthy of support through evaluation using the Foundation's intellectual merit and broader impacts review criteria.

该奖项全部或部分根据2021年美国救援计划法案（公法117-2）资助。非技术描述：材料对电场和磁场的响应方式决定了其在电子和光学设备中的功能和实用性。非线性过程允许具有广泛应用的有趣现象。例如，光限幅材料可以在低光强度下是透明的，但在高（且潜在危险）强度下是不透明的。这允许用户在正常条件下观看，同时保护他们免受伤害。非线性电磁材料可以满足对具有新功能和更高效率的设备日益增长的需求。这个CAREER项目旨在探索新形式的非线性电磁学，这些电磁学来自于新型二维量子材料中电子的量子特性。低维度产生了新的量子限制效应，可以实现用于信息和能源技术的高效和可调谐电子设备。PI将通过从层状2D材料中制造电子器件并研究其在低温下的非线性电磁响应来探索原子级薄层状量子材料的物理学。该项目紧密结合了研究活动，学生辅导，教育计划和以量子材料，物理和技术为中心的推广计划。首席研究员特别致力于通过促进女性研究人员和通过倡议计划培养年轻而充满活力的力量储备来解决物理学中的性别不平等问题。本项目由材料研究部（DMR）的电子和光子材料（EMPs）和凝聚态物理（CMP）项目共同资助。技术说明：非线性电磁响应是材料对外部电磁场的非线性响应现象。最近的进展揭示了非线性电磁响应与量子物质的拓扑和Berry曲率性质之间的深刻联系，导致拓扑非线性电磁学的新兴领域。在这一新生领域，有许多问题需要解决。例如，新拓扑状态的特征非线性响应是什么，它们能有多大？杂质和散射在这些过程中起什么作用？库仑相互作用的作用是什么？我们能用这些反应来探测和操纵涌现阶段吗？这个CAREER项目旨在通过探索原子级薄层量子材料的物理学来回答这些问题，这些量子材料具有可控的费米能量，能带结构，对称性，拓扑结构和电子相互作用，通过静电门控，货车德瓦尔斯堆叠和层扭曲。研究人员开发了创新的制造方法，从这些材料中创建可编程电子器件，并在具有宽带电磁激励的自制多功能磁传输/光学低温系统中研究其非线性电磁特性。将高度可调的非线性材料与宽带激发相结合，将允许在拓扑和相关材料中探索以前无法实现的领域。该奖项反映了NSF的法定使命，并通过使用基金会的知识价值和更广泛的影响审查标准进行评估，被认为值得支持。

项目成果

Quantum metric nonlinear Hall effect in a topological antiferromagnetic heterostructure

• DOI: 10.1126/science.adf1506
• 发表时间: 2023-06
• 期刊: Science
• 影响因子: 56.9
• 作者: Anyuan Gao;Yu-Fei Liu;Jian-Xiang Qiu;B. Ghosh;Thaís V Trevisan;Y. Onishi;Chaowei Hu;Tiema Qian;Hung-Ju Tien;Shaojuan Chen;Mengqi Huang;Damien Bérubé;Houchen Li;C. Tzschaschel;T. Dinh;Zhengyuan Sun;Sheng-Chin Ho;S. Lien;Bahadur Singh;Kenji Watanabe;T. Taniguchi;D. Bell;Hsin Lin;Tay-Rong Chang;C. Du;A. Bansil;L. Fu;Ni Ni-Ni;P. P. Orth-P.;Qiong Ma;Su-Yang Xu

Axion optical induction of antiferromagnetic order

• DOI: 10.1038/s41563-023-01493-5
• 发表时间: 2023-03
• 期刊: Nature Materials
• 影响因子: 41.2
• 作者: Jian-Xiang Qiu;C. Tzschaschel;J. Ahn;Anyuan Gao;Houchen Li;Xin-Yue Zhang;B. Ghosh;Chaowei Hu;Yu-Xuan Wang;Yu-Fei Liu;Damien Bérubé;T. Dinh;Zhenhao Gong;S. Lien;Sheng-Chin Ho;Bahadur Singh;Kenji Watanabe;T. Taniguchi;D. Bell;Hai-Zhou Lu;A. Bansil;Hsin Lin;Tay-Rong Chang;B. Zhou;Qiong Ma;A. Vishwanath;Ni Ni-Ni;Su-Yang Xu

Ultrathin GaN Crystal Realized Through Nitrogen Substitution of Layered GaS

• DOI: 10.1007/s11664-023-10670-w
• 发表时间: 2023-09
• 期刊: Journal of Electronic Materials
• 影响因子: 2.1
• 作者: Jun Cao;Tianshu Li;Hongze Gao;Xin Cong;Miao‐Ling Lin;Nicholas Russo;Weijun Luo;Siyuan Ding;Zifan Wang;Kevin E. Smith;Ping-Heng Tan;Qiong Ma;X. Ling