Ultrafast molecular stabilization mediated by electronic correlations (A07*)

该项目将使用阿秒时间分辨光谱学研究共轭电子系统中的电子关联，例如环状多碳分子。我们将专注于两个相互关联驱动的过程：第一，我们将与其他项目密切合作，研究突然电离分子中的电荷迁移；第二，我们将研究如何使用基于关联的机制，如抖动，在解离分子中实现激光稳定过程。

The project will investigate electronic correlations in conjugated electron systems such as cyclic polycarbon molecules using attosecond time resolved spectroscopy. We will focus on two correlation-driven processes: first we will investigate charge migration in suddenly ionized molecules - in close collaboration with other Projects - and secondly we will study how correlation-based mechanisms such as shake-up can be used to implement a laser stabilization process in the dissociative molecule.