Cyclotron resonance measurements of BEDT-TTF salts above the kink field under high field
Cyclotron resonance measurements of BEDT-TTF salts above the kink field under high field
批准号:
10440109
负责人:
OHTA Hitosi
金额:
$9.22万
依托单位:
依托单位国家:
日本
项目类别:
Grant-in-Aid for Scientific Research (B).
财政年份:
1998
资助国家:
日本
项目状态:
已结题
起止时间:
1998 至 2000
中文摘要
1.研制并安装了新型的3 kV 100 kJ电容器电源; 2.研制了Cu-Ag丝脉冲磁体,并利用新型的3 kV 100 kJ电容器组实现了36 T的低温超导磁体; 3.研制了一种新型的低温超导磁体,并在低温下进行了高场ESR测量。(2)利用这种新型低温恒温器,我们在1.8K下对二维有机导体α-(BEDT-TTF)_2KHg(SCN)_4进行了回旋共振测量,确定了扭结场下SDW相的四个有效质量:0.46m_e(CRI),0.96m_e(CR_2),1.30m_e(CR_3),1.71m_e(CR_4)。(3)我们成功地观察到回旋共振CR_3在1.8K的高场阶段以上的扭结场使用频率466-503 GHz。由于CR 3与α轨道的共振CR2不同,这一结果表明在高温相和高场相之间存在相边界。(BEDT-TTF)_2I_3的费米面比α-(BEDT-TTF)_2 KHg(SCN)_4,用矢量网络分析仪测量了样品的温度和模式耦合关系,确定了样品的有效质量分别为1.03m_e和2.14m_e。e.5我们用矢量网络分析仪观测了二维有机导体(BEDT-TTF)_2Br(DIA)在0.5K以下的回旋共振,观测到了5阶共振。观测到的共振可能是Hill等人提出的周期轨道共振,详细的分析正在进行中。
英文摘要
1 New power supply for the 3kV 100kJ capacitors was made and installed.2 We made a Cu-Ag wire pulsed magnet and achieved 36T using the new 3kV 100kJ capacitor bank.3(1) We made a new cryostat equiped with the 36T Cu-Ag pulsed magnet and made several high field ESR measurements at low temperature.(2) Using this new cryostat, we made cyclotron resonance measurements of two dimensional organic conductor α-(BEDT-TTF) _2 KHg (SCN) _4 at 1.8K.We determined 4 effective masses 0.46m_e (CRI), 0.96m_e (CR2), 1.30m_e (CR3), 1.71m_e (CR4) in the SDW phase below the kink field.(3) We succeeded in observing the cyclotron resonance CR3 at 1.8K in the high field phase above the kink field using the frequencies 466-503 GHz. As CR3 is different from the resonance CR2 from the α orbit, this result suggests that there exists a phase boundary between the high temperature phase and the high field phase.4 We observed the cyclotron resonances of θ-(BEDT-TTF) _2I_3, which has much simpler Fermi surface than α-(BEDT-TTF) _2 KHg (SCN) _4, by vector network analyzer down to 0.5K.We measured the temperature and the mode coupling dependences and determined the effective masses as 1.03m_e and 2.14m_e.5 We observed the cyclotron resonances of two dimensional or ganic conductor (BEDT-TTF) 2Br (DIA) by vector network analyzer down to 0.5 K.The resonances were observed up to 5th order. Observed resonances may be the periodic orbit resonance proposed by Hill et al. and the detailed analyses are on the way.
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H.Ohta: "High Frequency ESR Measurements Using Pulsed Magnetic Fields in Kobe"Physica B. (印刷中).
H. Ohta:“在神户使用脉冲磁场进行高频 ESR 测量”Physica B.(出版中)。
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K.Akioka: "Submillimeter Wave ESR Measurements of Two Dimensional Organic Antiferromagnet β'-(BEDT-TTF)_2lCl_2" J.Magn.Magn.Mater.177-181. 746-747 (1998)
K.Akioka:“二维有机反铁磁体 β-(BEDT-TTF)_2lCl_2 的亚毫米波 ESR 测量”J.Magn.Magn.Mater.177-181 (1998)。
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Y.Oshima: "Cyclotron Resonance Study of θ-(BEDT-TTF)_2I_3"Synthetic Metals. 103. 1919-1920 (1999)
Y.Oshima:“θ-(BEDT-TTF)_2I_3 的回旋共振研究”103. 1919-1920 (1999)
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N.Nakagawa: "X-band and Millimeter Wave ESR Studies of(DI-DCNQI)_2Ag" Synthetic Metals.
N.Nakakawa:“(DI-DCNQI)_2Ag 的 X 波段和毫米波 ESR 研究”合成金属。
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H.Ohta: "Circularly Polarized Cyclotron Resonance Measurement System and Its Application to BEDT-TTF Salts" Synthetic Metals.
H.Ohta:“圆偏振回旋共振测量系统及其在 BEDT-TTF 盐中的应用”合成金属。
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