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Mid-valent chromium reagents for controlled radical reactivity

Mid-valent chromium reagents for controlled radical reactivity
用于控制自由基反应性的中价铬试剂
批准号：
238716-2011
负责人：
Smith, Kevin
金额：
$2.55万
依托单位：
University of British Columbia
依托单位国家：
加拿大
项目类别：
Discovery Grants Program - Individual
财政年份：
2011
资助国家：
加拿大
项目状态：
已结题
起止时间：
2011-01-01 至 2012-12-31
来源：
https://www.nserc-crsng.gc.ca/ase-oro/Details-Detailles_eng.asp?id=478945
关键词：
Midvalentchromiumreagentscontrolled

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英文摘要
The catalytic use of transition metals has irrevocably changed the way chemists form carbon-carbon bonds, for applications from the synthesis of pharmaceuticals to the preparation of advanced materials. In the past five years, an increasing number of C-C bond forming reactions have been found to involve carbon-based radicals, highly reactive species that possess an unpaired electron. Many of these processes involve elements (e.g. first row transition metals, Ti-Cu) and/or ligands (e.g. diimines) that are known to be able to accommodate unpaired electrons. However, the relationship between optimal catalytic activity and the electronic structure of the reactive species is presently far from clear.
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